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  Mechanisms of the diterpene cyclases β-pinacene synthase from Dictyostelium discoideum and hydropyrene synthase from Streptomyces clavuligerus

Rinkel, J., Rabe, P., Chen, X., Köllner, T. G., Chen, F., & Dickschat, J. S. (2017). Mechanisms of the diterpene cyclases β-pinacene synthase from Dictyostelium discoideum and hydropyrene synthase from Streptomyces clavuligerus. Chemistry – A European Journal, 23(44), 10501-10505. doi:10.1002/chem.201702704.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-93C7-3 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-C3AC-6
Genre: Journal Article

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GER484s1.pdf (Supplementary material), 7MB
 
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 Creators:
Rinkel, Jan, Author
Rabe, Patrick, Author
Chen, Xinlu, Author
Köllner, Tobias G.1, Author           
Chen, Feng, Author
Dickschat, Jeroen S., Author
Affiliations:
1Department of Biochemistry, Prof. J. Gershenzon, MPI for Chemical Ecology, Max Planck Society, ou_421893              

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 Abstract: Two diterpene cyclases, one from the social amoeba Dictyostelium discoideum and the other from the bacterium Streptomyces clavuligerus, with products containing a Z-configured double bond between the original C2 and C3 of geranylgeranyl diphosphate, were extensively investigated for their mechanisms through isotopic labelling experiments. The participation of geranyllinalyl diphosphate, in analogy to the role of linalyl and nerolidyl diphosphate for mono- and sesquiterpene biosynthesis, as an intermediate towards diterpenes with a Z-configured C2=C3 double bond is discussed.

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 Dates: 2017-072017-07-112017-07-17
 Publication Status: Issued
 Pages: -
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 Table of Contents: -
 Rev. Type: -
 Identifiers: Other: GER484
DOI: 10.1002/chem.201702704
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Title: Chemistry – A European Journal
  Other : Chem. – Eur. J.
Source Genre: Journal
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Publ. Info: Weinheim, Germany : VCH Verlagsgesellschaft
Pages: - Volume / Issue: 23 (44) Sequence Number: - Start / End Page: 10501 - 10505 Identifier: ISSN: 0947-6539
CoNE: https://pure.mpg.de/cone/journals/resource/954926979058