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  Efficiency of Ni nanoparticles supported on hierarchical porous nitrogen-doped carbon for hydrogenolysis of Kraft lignin in flow and batch systems

Lama, S., Pampel, J., Fellinger, T.-P., Beškoski, V. P., Slavković-Beškoski, L., Antonietti, M., et al. (2017). Efficiency of Ni nanoparticles supported on hierarchical porous nitrogen-doped carbon for hydrogenolysis of Kraft lignin in flow and batch systems. ACS Sustainable Chemistry & Engineering, 5(3), 2415-2420. doi:10.1021/acssuschemeng.6b02761.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-41B3-D Version Permalink: https://hdl.handle.net/21.11116/0000-0007-F336-A
Genre: Journal Article

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 Creators:
Lama, Sandy1, Author           
Pampel, Jonas2, Author           
Fellinger, Tim-Patrick2, Author           
Beškoski, Vladimir P., Author
Slavković-Beškoski, Latinka, Author
Antonietti, Markus3, Author           
Molinari, Valerio4, 5, Author           
Affiliations:
1Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2364733              
2Tim Fellinger, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863322              
3Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              
4Davide Esposito, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863315              
5Valerio Molinari, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2385693              

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 Abstract: Ni nanoparticles supported on nitrogen-doped carbon (NDC) prepared via salt-melt synthesis with a hierarchical porosity were successfully applied as the catalyst for the degradation of Kraft lignin. It is shown that Ni-NDC is more efficient when compared to Ni nanoparticles deposited on an N-free carbon support, prepared with similar porosity features (Ni–C) and to Ni nanoparticles deposited on a commercial carbon (Ni-Cref). The efficiency of these materials was compared for reactions performed both in batch and flow reactors, highlighting the effect of the reactor setup on the stability of the recovered catalysts.

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 Dates: 2017
 Publication Status: Issued
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 Identifiers: DOI: 10.1021/acssuschemeng.6b02761
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Title: ACS Sustainable Chemistry & Engineering
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: 5 (3) Sequence Number: - Start / End Page: 2415 - 2420 Identifier: ISSN: 2168-0485