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  Single-atom control of the optoelectronic response in sub-nanometric cavities

Garcia-Gonzalez, P., Varas, A., Garcia-Vidal, F. J., & Rubio, A. (2019). Single-atom control of the optoelectronic response in sub-nanometric cavities.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0005-45A9-F Version Permalink: https://hdl.handle.net/21.11116/0000-0005-45AA-E
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1903.08443.pdf (Preprint), 3MB
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2019
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https://arxiv.org/abs/1903.08443 (Preprint)
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 Creators:
Garcia-Gonzalez, P.1, 2, Author
Varas, A.2, Author
Garcia-Vidal, F. J.1, 3, Author
Rubio, A.2, 4, 5, 6, 7, Author           
Affiliations:
1Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, ou_persistent22              
2Nano-Bio Spectroscopy Group and ETSF, Universidad del País Vasco UPV/EHU, ou_persistent22              
3Donostia International Physics Center (DIPC), ou_persistent22              
4Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
5Center for Free-Electron Laser Science, ou_persistent22              
6Department of Physics, University of Hamburg, ou_persistent22              
7Center for Computational Quantum Physics, Flatiron Institute, ou_persistent22              

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 Abstract: By means of ab-initio time dependent density functional theory calculations carried out on an prototypical hybrid plasmonic device (two metallic nanoparticles bridged by a one-atom junction), we demonstrate the strong interplay between photoinduced excitation of localized surface plasmons and electron transport through the single atom. Such an interplay is remarkably sensitive to the atomic orbitals of the junction. Therefore, we show the possibility of a twofold tuning (plasmonic response and photoinduced current across the juntion) just by changing a single atom in the device.

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Language(s): eng - English
 Dates: 2019-03-20
 Publication Status: Published online
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: arXiv: 1903.08443
 Degree: -

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