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  Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules.

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S. W., Cryle, M., et al. (2013). Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules. Physical Review Letters, 110(5): 053003. doi:10.1103/PhysRevLett.110.053003.

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 Creators:
Erk, B., Author
Rolles, D.1, Author              
Foucar, L., Author
Rudek, B., Author
Epp, S. W., Author
Cryle, M., Author
Bostedt, C., Author
Schorb, S., Author
Bozek, J., Author
Rouzee, A., Author
Hundertmark, A., Author
Marchenko, T., Author
Simon, M., Author
Filsinger, F., Author
Christensen, L., Author
De, S., Author
Trippel, S., Author
Kupper, J., Author
Stapelfeldt, H., Author
Wada, S., Author
Ueda, K., AuthorSwiggers, M., AuthorMesserschmidt, M., AuthorSchroter, C. D., AuthorMoshammer, R., AuthorSchlichting, I., AuthorUllrich, J., AuthorRudenko, A., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society, ou_578564              

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 Abstract: Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017  W/cm2) 5 fs x-ray pulses (ℏω=2  keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner-shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization.

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Language(s): eng - English
 Dates: 2013-01-302013-02-01
 Publication Status: Published in print
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 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.110.053003
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Title: Physical Review Letters
Source Genre: Journal
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Pages: 5 Volume / Issue: 110 (5) Sequence Number: 053003 Start / End Page: - Identifier: -