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  Role of virtual band population for high harmonic generation in solids

Sanari, Y., Hirori, H., Aharen, T., Tahara, H., Shinohara, Y., Ishikawa, K. L., et al. (2020). Role of virtual band population for high harmonic generation in solids. Physical Review B, 102(4): 041125(R). doi:10.1103/PhysRevB.102.041125.

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Datensatz-Permalink: https://hdl.handle.net/21.11116/0000-0006-D6B2-F Versions-Permalink: https://hdl.handle.net/21.11116/0000-0006-D6B3-E
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PhysRevB.102.041125.pdf (Verlagsversion), 3MB
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Supplemental Material: I. Synthesis of lead halide perovskite sample, II. HHG measurement, III. Theoretical method, IV. Evaluation of temporal population dynamics, V. Decomposition of calculated HHG spectra, VI. Rabi oscillation and virtual population dynamics, VII. Anisotropy of virtual population and high-order harmonic generation
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Sanari, Y.1, Autor
Hirori, H.1, Autor
Aharen, T.1, Autor
Tahara, H.1, Autor
Shinohara, Y.2, 3, Autor
Ishikawa, K. L.2, 3, 4, Autor
Otobe, T.5, Autor
Xia, P.6, Autor
Ishii, N.6, Autor
Itatani, J.6, Autor
Sato, S.7, 8, Autor           
Kanemitsu, Y.1, Autor
Affiliations:
1Institute for Chemical Research, Kyoto University, ou_persistent22              
2Photon Science Center, Graduate School of Engineering, The University of Tokyo, ou_persistent22              
3Department of Nuclear Engineering and Management, Graduate School of Engineering, The University of Tokyo, ou_persistent22              
4Research Institute for Photon Science and Laser Technology, The University of Tokyo, ou_persistent22              
5Kansai Photon Science Institute, National Institutes for Quantum and Radiological Science and Technology, ou_persistent22              
6Institute for Solid State Physics, The University of Tokyo, ou_persistent22              
7Center for Computational Sciences, University of Tsukuba, ou_persistent22              
8Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              

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 Zusammenfassung: We study the sub-band-gap high harmonic generation (HHG) in a methylammonium lead trichloride single crystal. Anisotropy in the crystal orientation dependence of the high harmonic yield is observed, and the yield varies substantially with the electric field strength of the midinfrared laser pulse used for excitation. Our real-time ab initio simulations reproduce the experimental results well and also show that the HHG is independent of the interband decoherence time. Based on a microscopic analysis of the intraband current, we reveal that the orientation dependence of the HHG in this perovskite semiconductor is governed by the virtual band population, rather than the anharmonicity of the electronic band structure.

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Sprache(n): eng - English
 Datum: 2020-05-012019-10-232020-07-132020-07-302020-07-15
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1103/PhysRevB.102.041125
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Titel: Physical Review B
  Kurztitel : Phys. Rev. B
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Woodbury, NY : American Physical Society
Seiten: - Band / Heft: 102 (4) Artikelnummer: 041125(R) Start- / Endseite: - Identifikator: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008