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  Time-resolved soft X-ray absorption spectroscopy in transmission mode on liquids at MHz repetition rates

Fondell, M., Eckert, S., Jay, R. M., Weniger, C., Quevedo, W., Niskanen, J., et al. (2017). Time-resolved soft X-ray absorption spectroscopy in transmission mode on liquids at MHz repetition rates. Structural Dynamics, 4(5): 054902. doi:10.1063/1.4993755.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0002-4F1C-8 Version Permalink: https://hdl.handle.net/21.11116/0000-0004-B811-9
Genre: Journal Article

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https://dx.doi.org/10.1063/1.4993755 (Publisher version)
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 Creators:
Fondell, M.1, Author
Eckert, S.2, Author
Jay, R. M.2, Author
Weniger, C.1, Author
Quevedo, W.1, Author
Niskanen, J.1, Author
Kennedy, B.1, Author
Sorgenfrei, F.2, Author
Schick, D.1, Author
Giangrisostomi, E.1, Author
Ovsyannikov, R.1, Author
Adamczyk, K.3, Author
Huse, N.4, Author           
Wernet, P.1, Author
Mitzner, R.1, Author
Föhlisch, A.1, 2, Author
Affiliations:
1Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin für Materialien und Energie, ou_persistent22              
2Institut für Physik und Astronomie, Universität Potsdam, ou_persistent22              
3Department of Physics, University of Hamburg and Center for Free-Electron Laser Science, ou_persistent22              
4Ultrafast Molecular Dynamics, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938289              

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 Abstract: We present a setup combining a liquid flatjet sample delivery and a MHz laser system for time-resolved soft X-ray absorption measurements of liquid samples at the high brilliance undulator beamline UE52-SGM at Bessy II yielding unprecedented statistics in this spectral range. We demonstrate that the efficient detection of transient absorption changes in transmission mode enables the identification of photoexcited species in dilute samples. With iron(II)-trisbipyridine in aqueous solution as a benchmark system, we present absorption measurements at various edges in the soft X-ray regime. In combination with the wavelength tunability of the laser system, the set-up opens up opportunities to study the photochemistry of many systems at low concentrations, relevant to materials sciences, chemistry, and biology.

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Language(s): eng - English
 Dates: 2017-06-302017-08-072017-08-142017-09
 Publication Status: Issued
 Pages: -
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 Rev. Type: Peer
 Identifiers: DOI: 10.1063/1.4993755
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Project name : We thank HZB for the allocation of synchrotron radiation beamtime. We thank Martin Beye, Mike Sperling, Karsten Holldack and Benjamin Dubrau for technical support during the measurements. D.S. acknowledges the Helmholtz Association for funding via the Helmholtz Postdoc Programme PD-142. S.E., R.J., F.S., and A.F. acknowledge funding from the ERC-ADG- 2014-Advanced Investigator Grant No. 669531 EDAX under the Horizon 2020 EU Framework Programme for Research and Innovation.
Grant ID : 669531
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

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Title: Structural Dynamics
Source Genre: Journal
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Publ. Info: Melville, NY : American Institute of Physics
Pages: - Volume / Issue: 4 (5) Sequence Number: 054902 Start / End Page: - Identifier: ISSN: 2329-7778
CoNE: https://pure.mpg.de/cone/journals/resource/2329-7778