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  Incommensurate spin correlations in highly oxidized cobaltates La2-xSrxCoO4

Li, Z. W., Drees, Y., Kuo, C. Y., Guo, H., Ricci, A., Lamago, D., et al. (2016). Incommensurate spin correlations in highly oxidized cobaltates La2-xSrxCoO4. Scientific Reports, 6: 25117, pp. 1-8. doi:10.1038/srep25117.

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Li, Z. W.1, Autor           
Drees, Y.1, Autor           
Kuo, C. Y.1, Autor           
Guo, H.1, Autor           
Ricci, A.2, Autor
Lamago, D.2, Autor
Sobolev, O.2, Autor
Ruett, U.2, Autor
Gutowski, O.2, Autor
Pi, T. W.2, Autor
Piovano, A.2, Autor
Schmidt, W.2, Autor
Mogare, K.3, Autor           
Hu, Z.4, Autor           
Tjeng, L. H.5, Autor           
Komarek, A. C.6, Autor           
Affiliations:
1Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863445              
2External Organizations, ou_persistent22              
3Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863425              
4Zhiwei Hu, Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863461              
5Liu Hao Tjeng, Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863452              
6Alexander Komarek, Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863446              

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 Zusammenfassung: We observe quasi-static incommensurate magnetic peaks in neutron scattering experiments on layered cobalt oxides La2-xSrxCoO4 with high Co oxidation states that have been reported to be paramagnetic. This enables us to measure the magnetic excitations in this highly hole-doped incommensurate regime and compare our results with those found in the low-doped incommensurate regime that exhibit hourglass magnetic spectra. The hourglass shape of magnetic excitations completely disappears given a high Sr doping. Moreover, broad low-energy excitations are found, which are not centered at the incommensurate magnetic peak positions but around the quarter-integer values that are typically exhibited by excitations in the checkerboard charge ordered phase. Our findings suggest that the strong inter-site exchange interactions in the undoped islands are critical for the emergence of hourglass spectra in the incommensurate magnetic phases of La2-xSrxCoO4.

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Sprache(n): eng - English
 Datum: 2016-04-27
 Publikationsstatus: Online veröffentlicht
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: ISI: 000374858800002
DOI: 10.1038/srep25117
 Art des Abschluß: -

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Titel: Scientific Reports
  Kurztitel : Sci. Rep.
Genre der Quelle: Zeitschrift
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Affiliations:
Ort, Verlag, Ausgabe: London, UK : Nature Publishing Group
Seiten: - Band / Heft: 6 Artikelnummer: 25117 Start- / Endseite: 1 - 8 Identifikator: Anderer: 2045-2322
CoNE: https://pure.mpg.de/cone/journals/resource/2045-2322