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  Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers

Rosenfeld, D., Zheng, Y., Hashimshoni, E., Pöhlker, M. L., Jefferson, A., Pöhlker, C., et al. (2016). Satellite retrieval of cloud condensation nuclei concentrations by using clouds as CCN chambers. Proceedings of the National Academy of Sciences of the United States of America, 113(21), 5828-5834. doi:10.1073/pnas.1514044113.

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Rosenfeld, Daniel1, Autor
Zheng, Youtong1, Autor
Hashimshoni, Eyal1, Autor
Pöhlker, M. L.2, Autor           
Jefferson, Anne1, Autor
Pöhlker, C.3, Autor           
Yu, Xing1, Autor
Zhu, Yannian1, Autor
Liu, Guihua1, Autor
Yue, Zhiguo1, Autor
Fischman, Baruch1, Autor
Li, Zhanqing1, Autor
Giguzin, David1, Autor
Goren, Tom1, Autor
Artaxo, Paulo1, Autor
Barbosa, Henrique M. J.1, Autor
Pöschl, U.2, Autor           
Andreae, M. O.3, Autor           
Affiliations:
1external, ou_persistent22              
2Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              
3Biogeochemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826286              

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 Zusammenfassung: Quantifying the aerosol/cloud-mediated radiative effect at a global scale requires simultaneous satellite retrievals of cloud condensation nuclei (CCN) concentrations and cloud base updraft velocities (W-b). Hitherto, the inability to do so has been a major cause of high uncertainty regarding anthropogenic aerosol/cloud-mediated radiative forcing. This can be addressed by the emerging capability of estimating CCN and W-b of boundary layer convective clouds from an operational polar orbiting weather satellite. Our methodology uses such clouds as an effective analog for CCN chambers. The cloud base supersaturation (S) is determined by W-b and the satellite-retrieved cloud base drop concentrations (N-db), which is the same as CCN(S). Validation against ground-based CCN instruments at Oklahoma, at Manaus, and onboard a ship in the northeast Pacific showed a retrieval accuracy of +/- 25% to +/- 30% for individual satellite overpasses. The methodology is presently limited to boundary layer not raining convective clouds of at least 1 km depth that are not obscured by upper layer clouds, including semi-transparent cirrus. The limitation for small solar backscattering angles of < 25 degrees restricts the satellite coverage to similar to 25% of the world area in a single day.

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Sprache(n): eng - English
 Datum: 2016
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: ISI: 000376779900039
DOI: 10.1073/pnas.1514044113
 Art des Abschluß: -

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Titel: Proceedings of the National Academy of Sciences of the United States of America
  Andere : Proc. Acad. Sci. USA
  Andere : Proc. Acad. Sci. U.S.A.
  Kurztitel : PNAS
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Washington, D.C. : National Academy of Sciences
Seiten: - Band / Heft: 113 (21) Artikelnummer: - Start- / Endseite: 5828 - 5834 Identifikator: ISSN: 0027-8424
CoNE: https://pure.mpg.de/cone/journals/resource/954925427230