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  Gold catalysis meets materials science – a new approach to pi‐extended indolocarbazoles

Hendrich, C., Bongartz, L. M., Hoffmann, M., Zschieschang, U., Borchert, J. W., Sauter, D., et al. (2020). Gold catalysis meets materials science – a new approach to pi‐extended indolocarbazoles. Advanced Synthesis & Catalysis, 1-10. doi:10.1002/adsc.202001123.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0007-59EB-D Version Permalink: https://hdl.handle.net/21.11116/0000-0007-59EC-C
Genre: Journal Article

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 Creators:
Hendrich, Christoph, Author
Bongartz, Lukas M., Author
Hoffmann, Marvin, Author
Zschieschang, Ute, Author
Borchert, James W., Author
Sauter, Désirée1, Author           
Krämer, Petra, Author
Rominger, Frank, Author
Mulks, Florian F., Author
Rudolph, Matthias, Author
Dreuw, Andreas, Author
Klauk, Hagen, Author
Hashmi, A. Stephen K., Author
Affiliations:
1Cellular Biophysics, Max Planck Institute for Medical Research, Max Planck Society, ou_2364731              

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Free keywords: thin-film transistors; indolocarbazoles; Materials science; organic semiconductors; gold catalysis; modular synthesis
 Abstract: Herein we describe a modular, convergent synthesis of substituted benzo[a]benzo[6,7]‐indolo[2,3‐h]carbazoles (BBICZs) using a bidirectional gold‐catalyzed cyclization reaction as a key step. A building block strategy enabled the easy variation of substituents at different positions of the core structure and a general analysis of substitution effects on the materials properties of the target compounds. All BBICZs were fully characterized and their optical and electronic properties were studied experimentally as well as by computational methods. Organic thin‐film transistors based on eight selected derivatives were fabricated by vacuum deposition and charge‐carrier mobilities up to 1 cm2/Vs were measured.

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Language(s): eng - English
 Dates: 2020-11-02
 Publication Status: Published online
 Pages: 11
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/adsc.202001123
 Degree: -

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Title: Advanced Synthesis & Catalysis
  Abbreviation : Adv. Synth. Catal.
Source Genre: Journal
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Publ. Info: Weinheim, Fed. Rep. of Germany : Wiley-VCH Verlag GmbH
Pages: - Volume / Issue: - Sequence Number: - Start / End Page: 1 - 10 Identifier: ISSN: 1615-4150
CoNE: https://pure.mpg.de/cone/journals/resource/958634688013