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  Steady-state and forced periodic operation of solid electrolyte membrane reactors for selective oxidation of n-butane to maleic anhydride

Munder, B., Rihko-Struckmann, L., & Sundmacher, K. (2007). Steady-state and forced periodic operation of solid electrolyte membrane reactors for selective oxidation of n-butane to maleic anhydride. Chemical Engineering Science, 62(18-20 ), 5663-5668. doi:10.1016/j.ces.2007.01.042.

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Datensatz-Permalink: https://hdl.handle.net/11858/00-001M-0000-0013-9919-A Versions-Permalink: https://hdl.handle.net/11858/00-001M-0000-0027-8334-4
Genre: Zeitschriftenartikel

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 Urheber:
Munder, Barbara1, Autor           
Rihko-Struckmann, Liisa1, Autor           
Sundmacher, Kai1, 2, Autor           
Affiliations:
1Process Systems Engineering, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, ou_1738151              
2Otto-von-Guericke-Universität Magdeburg, External Organizations, ou_1738156              

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 Zusammenfassung: Experimental results obtained with a bilayer-solid electrolyte membrane reactor (bilayer-SEMR) are analysed based on a 1D+1D reactor model and attainable yields in steady-state and forced-periodic operation modes are determined. Optimal steady-state operation conditions are predicted in the range of high Damköhler numbers and oxidizing conditions. Forced-periodic operation of bilayer-SEMRs, which is easily established via the electric current, leads to a significant selectivity enhancement, but has to be critically rated with respect to energy expenses needed under electrochemical-oxygen-pumping conditions. copyright 2007 Elsevier Ltd. All rights reserved. [accessed February 8th 2013]

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Sprache(n): eng - English
 Datum: 2007
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: eDoc: 281003
Anderer: 12/07
DOI: 10.1016/j.ces.2007.01.042
 Art des Abschluß: -

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Titel: Chemical Engineering Science
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: -
Seiten: - Band / Heft: 62 (18-20 ) Artikelnummer: - Start- / Endseite: 5663 - 5668 Identifikator: -