Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple 
ionization of small polyatomic molecules

Erk, Benjamin; Rolles, Daniel; Foucar, Lutz; Rudek, Benedikt; Epp, Sascha; Cryle, Max; Bostedt, Christoph; Schorb, Sebastian; Bozek, John D.; Rouzee, Arnaud; Hundertmark, Axel; Marchenko, Tatiana; Simon, Marc; Filsinger, Frank; Christensen, Lauge; De, Shankar; Trippel, Sebastian; Küpper, Jochen; Stapelfeldt, Henrik; Wada, Shinichi; Ueda, Kiyoshi; Swiggers, Michelle L.; Messerschmidt, Marc; Schroeter, Claus-Dieter; Moshammer, Robert; Schlichting, Ilme; Ullrich, Joachim; Rudenko, Artem

doi:10.1103/PhysRevLett.110.053003

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Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S., Cryle, M., et al. (2013). Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules. Physical Review Letters, 110(5): 53003, pp. 1-5. doi:10.1103/PhysRevLett.110.053003.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-F218-6 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-002D-F219-4

Genre: Journal Article

Alternative Title : Ultrafast charge rearrangement and nuclear dynamics upon inner-shell multiple ionization of small polyatomic molecules

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Creators:
Erk, Benjamin¹, Author
Rolles, Daniel¹, Author
Foucar, Lutz¹, Author
Rudek, Benedikt¹, Author
Epp, Sascha², Author
Cryle, Max¹, Author
Bostedt, Christoph, Author
Schorb, Sebastian, Author
Bozek, John D., Author
Rouzee, Arnaud, Author
Hundertmark, Axel, Author
Marchenko, Tatiana, Author
Simon, Marc, Author
Filsinger, Frank, Author
Christensen, Lauge, Author
De, Shankar, Author
Trippel, Sebastian, Author
Küpper, Jochen, Author
Stapelfeldt, Henrik, Author
Wada, Shinichi, Author
Ueda, Kiyoshi, AuthorSwiggers, Michelle L., AuthorMesserschmidt, Marc, AuthorSchroeter, Claus-Dieter, AuthorMoshammer, Robert, AuthorSchlichting, Ilme¹, AuthorUllrich, Joachim, AuthorRudenko, Artem, Author more..

Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700
2Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284

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Abstract: Ionization and fragmentation of methylselenol (CH(3)SeH) molecules by intense (>10(17) W/cm(2)) 5 fs x-ray pulses (ħω=2 keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner-shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization.

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Language(s): eng - English

Dates: Submitted: 2012-10-02Accepted: 2013-01-30Published Online: 2013-01-30Date issued: 2013-02-01

Publication Status: Issued

Pages: 5

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Table of Contents: -

Rev. Type: Peer

Identifiers: eDoc: 664313
DOI: 10.1103/PhysRevLett.110.053003
URI: http://www.ncbi.nlm.nih.gov/pubmed/23414017
Other: 7882

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Title: Physical Review Letters

Other : Phys. Rev. Lett.

Source Genre: Journal

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Publ. Info: Woodbury, N.Y. : American Physical Society

Pages: - Volume / Issue: 110 (5) Sequence Number: 53003 Start / End Page: 1 - 5 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1