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  A quantitative comparison of time-of-flight momentum microscopes and hemispherical analyzers for time- and angle-resolved photoemission spectroscopy experiments

Maklar, J., Dong, S., Beaulieu, S., Pincelli, T., Dendzik, M. R., Windsor, Y. W., et al. (2020). A quantitative comparison of time-of-flight momentum microscopes and hemispherical analyzers for time- and angle-resolved photoemission spectroscopy experiments. Review of Scientific Instruments, 91(12): 123112. doi:10.1063/5.0024493.

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 Creators:
Maklar, Julian1, Author           
Dong, Shuo1, Author           
Beaulieu, Samuel1, Author           
Pincelli, Tommaso1, Author           
Dendzik, Maciej Ramon1, 2, Author           
Windsor, Yaov William1, Author           
Xian, R. Patrick1, 3, Author           
Wolf, Martin1, Author           
Ernstorfer, Ralph1, Author           
Rettig, Laurenz1, Author           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Department of Applied Physics, KTH Royal Institute of Technology, SE-16440 Stockholm, Kista, Sweden., ou_persistent22              
3Department of Neurobiology, Northwestern University, Evanston, Illinois 60208, USA., ou_persistent22              

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 Abstract: Time-of-flight-based momentum microscopy has a growing presence in photoemission studies, as it enables parallel energy- and momentum-resolved acquisition of the full photoelectron distribution. Here, we report table-top extreme ultraviolet time- and angle-resolved photoemission spectroscopy (trARPES) featuring both a hemispherical analyzer and a momentum microscope within the same setup. We present a systematic comparison of the two detection schemes and quantify experimentally relevant parameters, including pump- and probe-induced space-charge effects, detection efficiency, photoelectron count rates, and depth of focus. We highlight the advantages and limitations of both instruments based on exemplary trARPES measurements of bulk WSe2. Our analysis demonstrates the complementary nature of the two spectrometers for time-resolved ARPES experiments. Their combination in a single experimental apparatus allows us to address a broad range of scientific questions with trARPES.

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Language(s): eng - English
 Dates: 2020-08-072020-11-262021-12-222020-12
 Publication Status: Issued
 Pages: 11
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1063/5.0024493
 Degree: -

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Project name : FLATLAND - Electron-lattice-spin correlations and many-body phenomena in 2D semiconductors and related heterostructures
Grant ID : 682843
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

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Title: Review of Scientific Instruments
  Abbreviation : Rev. Sci. Instrum.
Source Genre: Journal
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Publ. Info: Melville, NY : AIP Publishing
Pages: 11 Volume / Issue: 91 (12) Sequence Number: 123112 Start / End Page: - Identifier: ISSN: 0034-6748
CoNE: https://pure.mpg.de/cone/journals/resource/991042742033452