English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT
 
 
DownloadE-Mail
 DetailsSummary
  Polarization-state-resolved high-harmonic spectroscopy of solids

Klemke, N., Tancogne-Dejean, N., Rossi, G. M., Yang, Y., Scheiba, F., Mainz, R. E., et al. (2019). Polarization-state-resolved high-harmonic spectroscopy of solids. Nature Communications, 10: 1319. doi:10.1038/s41467-019-09328-1.

Item is

 

show all hide all

Basic

show hide
Item Permalink: https://hdl.handle.net/21.11116/0000-0002-4E5E-F Version Permalink: https://hdl.handle.net/21.11116/0000-0005-5E16-A
Genre: Journal Article

Files

show Files
hide Files
:
s41467-019-09328-1.pdf (Publisher version), 2MB
View   Save
File Permalink:
https://hdl.handle.net/21.11116/0000-0003-3956-D
Name:
s41467-019-09328-1.pdf
Description:
This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.
OA-Status:
Not specified
Visibility:
Public
MIME-Type / Checksum:
application/pdf / [MD5]
Technical Metadata:
View
Copyright Date:
2019
Copyright Info:
© the Author(s)
License:
https://creativecommons.org/licenses/by/4.0/
:
41467_2019_9328_MOESM1_ESM.pdf (Supplementary material), 4MB
View   Save
File Permalink:
https://hdl.handle.net/21.11116/0000-0003-3957-C
Name:
41467_2019_9328_MOESM1_ESM.pdf
Description:
Supplementary Information
OA-Status:
Not specified
Visibility:
Public
MIME-Type / Checksum:
application/pdf / [MD5]
Technical Metadata:
View
Copyright Date:
2019
Copyright Info:
© the Author(s)
License:
-
:
41467_2019_9328_MOESM2_ESM.pdf (Supplementary material), 69KB
View   Save
File Permalink:
https://hdl.handle.net/21.11116/0000-0003-3958-B
Name:
41467_2019_9328_MOESM2_ESM.pdf
Description:
Peer Review File
OA-Status:
Not specified
Visibility:
Public
MIME-Type / Checksum:
application/pdf / [MD5]
Technical Metadata:
View
Copyright Date:
-
Copyright Info:
-
License:
-

Locators

show
hide
Locator:
https://arxiv.org/abs/1805.10453 (Preprint)
Description:
-
OA-Status:
Not specified
Locator:
https://dx.doi.org/10.1038/s41467-019-09328-1 (Publisher version)
Description:
-
OA-Status:
Not specified

Creators

show
hide
 Creators:
Klemke, N.1, 2, Author
Tancogne-Dejean, N.1, 3, Author           
Rossi, G. M.1, 2, Author
Yang, Y.1, 2, Author
Scheiba, F.1, 2, Author
Mainz, R. E.1, 2, Author
Di Sciacca, G.1, Author
Rubio, A.1, 2, 3, 4, 5, Author           
Kärtner, F. X.1, 2, 4, Author
Mücke, O. D.1, 4, Author
Affiliations:
1Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
2Physics Department, University of Hamburg, ou_persistent22              
3Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
4The Hamburg Centre for Ultrafast Imaging, ou_persistent22              
5Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              

Content

show
hide
Free keywords: -
 Abstract: Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the fast carrier dynamics in crystals holds great promise for next-generation petahertz electronics and devices. The carrier dynamics can produce high-order harmonics of the driving field extending up into the extreme-ultraviolet region. Here, we introduce polarization-state-resolved high-harmonic spectroscopy of solids, which provides deeper insights into both electronic and structural sub-cycle dynamics. Performing high-harmonic generation measurements from silicon and quartz, we demonstrate that the polarization states of the harmonics are not only determined by crystal symmetries, but can be dynamically controlled, as a consequence of the intertwined interband and intraband electronic dynamics. We exploit this symmetry-dynamics duality to efficiently generate coherent circularly polarized harmonics from elliptically polarized pulses. Our experimental results are supported by ab-initio simulations, providing evidence for the microscopic origin of the phenomenon.

Details

show
hide
Language(s): eng - English
 Dates: 2019-01-172019-03-012019-03-21
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: arXiv: 1805.10453
DOI: 10.1038/s41467-019-09328-1
 Degree: -

Event

show

Legal Case

show

Project information

show hide
Project name : We acknowledge support by the cluster of excellence “Advanced Imaging of Matter” (EXC 2056—project ID 390715994) and the priority program QUTIF (SPP1840 SOLSTICE) of the Deutsche Forschungsgemeinschaft, as well as financial support from the European Research Council (ERC-2015-AdG-694097), Grupos Consolidados (IT578-13), and European Union’s H2020 program under GA no. 676580 (NOMAD). N.T.-D., A.R., and O.D.M. thank M. Altarelli for very fruitful discussion. We thank M. Spiwek for help with the Laue X-ray diffraction characterization of samples.
Grant ID : 676580
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

Source 1

show
hide
Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 10 Sequence Number: 1319 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723