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  Structure Determination of Anionic Metal Clusters via Infrared Resonance Enhanced Multiple Photon Electron Detachment Spectroscopy

Haertelt, M., Lapoutre, V. J., Bakker, J. M., Redlich, B., Harding, D. J., Fielicke, A., et al. (2011). Structure Determination of Anionic Metal Clusters via Infrared Resonance Enhanced Multiple Photon Electron Detachment Spectroscopy. The Journal of Physical Chemistry Letters, 2, 1720-1724. doi:10.1021/jz200771w.

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 Creators:
Haertelt, Marko1, Author           
Lapoutre, Vivike J.2, Author
Bakker, Joost M.2, Author           
Redlich, Britta2, Author
Harding, Daniel J.1, Author           
Fielicke, André1, Author           
Meijer, Gerard1, Author           
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1Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
2FOM Institute for Plasma Physics Rijnhuizen, Edisonbaan 14, NL-3439 MN Nieuwegein, The Netherlands , ou_persistent22              

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 Abstract: We report vibrational spectra of anionic metal clusters, measured via electron detachment following resonant absorption of multiple infrared photons. To facilitate the sequential absorption of the required large number of photons, the cluster beam interacts with the infrared radiation inside the cavity of a free electron laser. Far-infrared spectra of the bare metal cluster anion Nb 10- as well as of the Nb 6C- anion are measured in the 130–1000 cm-1 range. The structures of these clusters can be unambiguously determined by comparison with calculated spectra of the putative global minima structures, identified by density functional theory calculations.

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Language(s): eng - English
 Dates: 20112011-06-282011-07
 Publication Status: Issued
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 Rev. Type: Peer
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Title: The Journal of Physical Chemistry Letters
  Other : J. Phys. Chem. Lett.
Source Genre: Journal
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Publ. Info: Columbus, OH : American Chemical Society
Pages: - Volume / Issue: 2 Sequence Number: - Start / End Page: 1720 - 1724 Identifier: ISSN: 1089-5639
CoNE: https://pure.mpg.de/cone/journals/resource/954926947766_4