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  Structural Identification of Caged Vanadium Doped Silicon Clusters

Claes, P., Janssens, E., Ngan, V. T., Gruene, P., Lyon, J. T., Harding, D. J., et al. (2011). Structural Identification of Caged Vanadium Doped Silicon Clusters. Physical Review Letters, 107(17): 173401. doi:10.1103/PhysRevLett.107.173401.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0012-2E38-3 Version Permalink: https://hdl.handle.net/21.11116/0000-0005-B9D2-D
Genre: Journal Article

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 Creators:
Claes, Pieterjan1, Author
Janssens, E.1, Author
Ngan, V. T.2, Author
Gruene, Philipp3, Author           
Lyon, Jonathan T.3, Author           
Harding, Daniel J.3, Author           
Fielicke, André3, Author           
Nguyen, M. T.2, Author
Lievens, P.1, Author
Affiliations:
1Laboratory of Solid State Physics and Magnetism, Katholieke Universiteit Leuven, Celestijnenlaan 200D, B-3001 Leuven, Belgium, ou_persistent22              
2Department of Chemistry, Katholieke Universiteit Leuven, Celestijnenlaan 200F, B-3001 Leuven, Belgium, ou_persistent22              
3Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              

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 Abstract: The geometry of cationic silicon clusters doped with vanadium, SinV⁺ (n=12–16), is investigated by using infrared multiple photon dissociation of the corresponding rare gas complexes in combination with ab initio calculations. It is shown that the clusters are endohedral cages, and evidence is provided that Si16V⁺ is a fluxional system with a symmetric Frank-Kasper geometry.

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Language(s): eng - English
 Dates: 2011-04-062011-10-172011-10-17
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.107.173401
URI: http://link.aps.org/doi/10.1103/PhysRevLett.107.173401
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Title: Physical Review Letters
  Other : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 107 (17) Sequence Number: 173401 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406