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  Making the Best of Mixed-Field Orientation of Polar Molecules: A Recipe for Achieving Adiabatic Dynamics in an Electrostatic Field Combined with Laser Pulses

Nielsen, J. H., Stapelfeldt, H., Küpper, J., Friedrich, B., Omiste, J., & Gonzales-Ferez, R. (2012). Making the Best of Mixed-Field Orientation of Polar Molecules: A Recipe for Achieving Adiabatic Dynamics in an Electrostatic Field Combined with Laser Pulses. Physical Review Letters, 108(19): 193001. doi:10.1103/PhysRevLett.108.193001.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-000F-4406-7 Version Permalink: https://hdl.handle.net/21.11116/0000-0005-E743-B
Genre: Journal Article

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 Creators:
Nielsen, Jens H.1, Author
Stapelfeldt, Henrik2, 3, Author
Küpper, Jochen4, 5, 6, Author           
Friedrich, Bretislav6, Author           
Omiste, J.J.7, Author
Gonzales-Ferez, R.7, Author
Affiliations:
1Department of Physics and Astronomy, University of Aarhus, 10.1039/C1CP21143A, ou_persistent22              
2Department of Chemistry, University of Aarhus, 8000 Aarhus C, Denmark, ou_persistent22              
3Interdisciplinary Nanoscience Center (iNANO), University of Aarhus, 8000 Aarhus C, Denmark, ou_persistent22              
4Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany, ou_persistent22              
5University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              
6Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
7Instituto Carlos I de Fısica Teorica y Computacional and Departamento de Fısica Atomica, Molecular y Nuclear, Universidad de Granada, 18071 Granada, Spain, ou_persistent22              

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 Abstract: We have experimentally and theoretically investigated the mixed-field orientation of rotational-stateselected
OCS molecules and achieved strong degrees of alignment and orientation. The applied
moderately intense nanosecond laser pulses are long enough to adiabatically align molecules.
However, in combination with a weak dc electric field, the same laser pulses result in nonadiabatic
dynamics of the mixed-field orientation. These observations are fully explained by calculations employing
both adiabatic and nonadiabatic (time-dependent) models

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Language(s): eng - English
 Dates: 2012-012012-012012-05-072012-05-07
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.108.193001
URI: http://link.aps.org/doi/10.1103/PhysRevLett.108.193001
 Degree: -

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Title: Physical Review Letters
  Other : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 108 (19) Sequence Number: 193001 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406