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  Hydrogen Production by Methanol Steam Reforming on Copper Boosted by Zinc-Assisted Water Activation

Rameshan, C., Stadlmayr, W., Penner, S., Lorenz, H., Memmel, N., Hävecker, M., et al. (2012). Hydrogen Production by Methanol Steam Reforming on Copper Boosted by Zinc-Assisted Water Activation. Angewandte Chemie International Edition: a journal of the Gesellschaft Deutscher Chemiker, 51(12), 3002-3006. doi:10.1002/anie.201106591.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-515F-7 Version Permalink: http://hdl.handle.net/21.11116/0000-0005-BEE1-7
Genre: Journal Article

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 Creators:
Rameshan, Christoph1, 2, Author              
Stadlmayr, Werner1, Author
Penner, Simon1, Author
Lorenz, Harald1, Author
Memmel, Norbert1, Author
Hävecker, Michael2, Author              
Blume, Raoul2, Author              
Teschner, Detre2, Author              
Rocha, Tulio2, Author              
Zemlyanov, Dmitry3, Author
Knop-Gericke, Axel2, Author              
Schlögl, Robert2, Author              
Klötzer, Bernhard1, Author
Affiliations:
1Institute of Physical Chemistry, University of Innsbruck, Innrain 52A, 6020 Innsbruck (Austria), ou_persistent22              
2Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
3Birck Nanotechnology Center, Purdue University,, 1205 West State Street, West Lafayette, IN 47907-2057 (USA), ou_persistent22              

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Free keywords: copper/zinc alloys; methanol steam reforming; surface chemistry; water activation; X-ray photoelectron spectroscopy
 Abstract: A Zn-in-Cu near-surface alloy covered by a thin wetting layer of interfacial Zn(ox) is the most active state of an inverse CuZn catalyst. The bifunctional action of the mixed Cu(Zn)0/Zn(ox) surface allows for selective dehydrogenation of methanol to formaldehyde and for optimized water activation, thus providing the required source of oxygen for the total oxidation of HCHO to CO2.

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Language(s): eng - English
 Dates: 2012-02-152012-03-19
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201106591
 Degree: -

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Title: Angewandte Chemie International Edition : a journal of the Gesellschaft Deutscher Chemiker
Source Genre: Journal
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Publ. Info: Weinheim/Bergstr. : Verlag Chemie
Pages: - Volume / Issue: 51 (12) Sequence Number: - Start / End Page: 3002 - 3006 Identifier: ISSN: 0570-0833
CoNE: https://pure.mpg.de/cone/journals/resource/110984073528720