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  Butadiene rubbers: topological constraints and microscopic deformation by mechanical and small angle neutron scattering investigation

Menge, H., Pyckhout-Hintzen, W., Meier, G., & Straube, E. (2002). Butadiene rubbers: topological constraints and microscopic deformation by mechanical and small angle neutron scattering investigation. Polymer Bulletin, 48(2), 183-190.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-663A-7 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-663B-5
Genre: Journal Article

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 Creators:
Menge, H., Author
Pyckhout-Hintzen, W., Author
Meier, G.1, Author              
Straube, E., Author
Affiliations:
1MPI for Polymer Research, Max Planck Society, ou_1309545              

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 Abstract: Results of stress-strain measurements are reported for butadiene rubbers of varying crosslink density. The fluctuation of the effective tube diameter of the polymer networks was investigated under uniaxial elongation by mechanical measurements as well as by small angle neutron scattering (SANS) which probe the local orientation on a segmental scale. The effect of topological constraints on the microscopic deformation of the butadiene network chains is well described within a tube approach. For the first time, experiments at large deformations and for polydisperse sample are presented. Excellent agreement between the statistical mechanical model and the experimental results is obtained.

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Language(s): eng - English
 Dates: 2002-04
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: eDoc: 28483
ISI: 000175608800011
 Degree: -

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Title: Polymer Bulletin
  Alternative Title : Polym. Bull.
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: -
Pages: - Volume / Issue: 48 (2) Sequence Number: - Start / End Page: 183 - 190 Identifier: ISSN: 0170-0839