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  Metallocene‐Catalyzed C7‐Linkage in the Hydrooligomerization of Norbornene by σ‐Bond Metathesis: Insight into the Microstructure of Polynorbornene

Karafilidis, C., Hermann, H., Rufiñska, A., Gabor, B., Mynott, R. J., Breitenbruch, G., et al. (2004). Metallocene‐Catalyzed C7‐Linkage in the Hydrooligomerization of Norbornene by σ‐Bond Metathesis: Insight into the Microstructure of Polynorbornene. Angewandte Chemie International Edition, 43(18), 2444-2446. doi:10.1002/anie.200353454.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-000F-9767-5 Version Permalink: https://hdl.handle.net/21.11116/0000-0007-51F1-D
Genre: Journal Article

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 Creators:
Karafilidis, Christos1, Author           
Hermann, Holger2, Author           
Rufiñska, Anna3, Author           
Gabor, Barbara3, Author           
Mynott, Richard J.3, Author           
Breitenbruch, Georg4, Author           
Weidenthaler, Claudia5, Author           
Rust, Jörg6, Author           
Joppek, Werner7, Author           
Brookhart, Maurice S.8, Author
Thiel, Walter2, Author           
Fink, Gerhard1, Author           
Affiliations:
1Research Department Fink, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445583              
2Research Department Thiel, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445590              
3Service Department Mynott (NMR), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445627              
4Service Department Belder (GC, HPLC), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_persistent22              
5Research Department Schüth, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445589              
6Service Department Lehmann (EMR), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445625              
7Service Department Schrader (MS), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445629              
8Department of Chemistry, University of North Carolina at Chapel Hill, CB#3290, Chapel Hill, NC 27599‐3290, USA, ou_persistent22              

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Free keywords: density functional calculations; metathesis; oligomerization; polynorbornene; zirconocene
 Abstract: An unusual linkage: The zirconocene‐catalyzed hydrooligomerization of norbornene proceeds by σ‐bond metathesis to form a 2‐exo,7′‐syn linkage (as evident in the pentamer shown). The oligomers were characterized by gas chromatography, NMR spectroscopy , X‐ray crystallography, and DFT calculations.

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Language(s): eng - English
 Dates: 2003-12-032004-04-222004-04-26
 Publication Status: Issued
 Pages: 3
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.200353454
 Degree: -

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Title: Angewandte Chemie International Edition
  Abbreviation : Angew. Chem., Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 43 (18) Sequence Number: - Start / End Page: 2444 - 2446 Identifier: ISSN: 1433-7851
CoNE: https://pure.mpg.de/cone/journals/resource/1433-7851