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  Time-resolved near-edge x-ray absorption fine structure spectroscopy on photo-induced phase transitions using a tabletop soft-x-ray spectrometer.

Grossmann, P., Pohl, J., Rajkovic, I., Barkusky, F., Jooss, V., Techert, S., et al. (2012). Time-resolved near-edge x-ray absorption fine structure spectroscopy on photo-induced phase transitions using a tabletop soft-x-ray spectrometer. Review of Scientific Instruments, 83(5): 053110. doi:10.1063/1.4718936.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-A0D9-2 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0028-9161-1
Genre: Journal Article

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1479037.pdf (Publisher version), 2MB
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Grossmann, P., Author
Pohl, J., Author
Rajkovic, I.1, Author              
Barkusky, F., Author
Jooss, V., Author
Techert, S.1, Author              
Mann, K., Author
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1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for biophysical chemistry, Max Planck Society, ou_578564              

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 Abstract: We present a table-top soft-x-ray spectrometer for the wavelength range λ = 1–5 nm based on a stable laser-driven x-ray source, making use of a gas-puff target. With this setup, optical light- pump/soft-x-ray probe near-edge x-ray absorption fine structure (NEXAFS) experiments with a temporal resolution of about 230 ps are feasible. Pump-probe NEXAFS measurements were car- ried out in the “water-window” region (2.28 nm–4.36 nm) on the manganite Pr 0.7 Ca 0.3 MnO 3 , investigating diminutive changes of the oxygen K edge that derive from an optically induced phase transition. The results show the practicability of the table-top soft-x-ray spectrometer on demand- ing investigations so far exclusively conducted at synchrotron radiation sources.

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Language(s): eng - English
 Dates: 2012-05-17
 Publication Status: Published online
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 Rev. Method: Peer
 Identifiers: DOI: 10.1063/1.4718936
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Title: Review of Scientific Instruments
Source Genre: Journal
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Pages: - Volume / Issue: 83 (5) Sequence Number: 053110 Start / End Page: - Identifier: -