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  Production of a beam of highly vibrationally excited CO using perturbations.

Bartels, N., Schäfer, T., Hühnert, J., Field, R. W., & Wodtke, A. M. (2012). Production of a beam of highly vibrationally excited CO using perturbations. The Journal of Chemical Physics, 136(21): 214201. doi:10.1063/1.4722090.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-A7F6-4 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0028-948B-B
Genre: Journal Article

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Bartels, N.1, Author              
Schäfer, T.1, Author              
Hühnert , J., Author
Field, R. W., Author
Wodtke, A. M.1, Author              
Affiliations:
1Department of Dynamics at Surfaces, MPI for biophysical chemistry, Max Planck Society, ou_578600              

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 Abstract: An intense molecular beam of CO ( X 1 + ) in high vibrational states ( v = 17, 18) was produced by a new approach that we call PUMP – PUMP – PERTURB and DUMP . The basic idea is to access high vibrational states of CO e 3 − via a two-photon doubly resonant transition that is per- turbed by the A 1 state. DUMP -ing from this mixed (predominantly triplet) state allows access to high vibrational levels of CO ( X 1 + ). The success of the approach, which avoids the use of vacuum UV radiation in any of the excitation steps, is proven by laser induced fluorescence and resonance enhanced multi-photon ionization spectroscopy.

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Language(s): eng - English
 Dates: 2012-06-052012
 Publication Status: Published in print
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 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1063/1.4722090
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Title: The Journal of Chemical Physics
Source Genre: Journal
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Pages: - Volume / Issue: 136 (21) Sequence Number: 214201 Start / End Page: - Identifier: ISSN: 1520-9032
CoNE: /journals/resource/991042752807952