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  White-light-induced fragmentation of toluene

Müller, A. M., Witzel, B., Uiterwaal, C. J. G. J., Wanner, J., & Kompa, K.-L. (2002). White-light-induced fragmentation of toluene. Physical Review Letters, 88(2): 023001. 023001. Retrieved from http://link.aps.org/abstract/PRL/v88/e023001.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-C269-1 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-000F-C26A-0
Genre: Journal Article

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 Creators:
Müller, Astrid M.1, Author              
Witzel, Bernd, Author
Uiterwaal, C. J. G. J.1, Author              
Wanner, Jochen1, Author              
Kompa, Karl-Ludwig1, Author              
Affiliations:
1Laser Chemistry, Max Planck Institute of Quantum Optics, Max Planck Society, ou_1445565              

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 Abstract: We investigate the influence of continuum generation on the photofragmentation dynamics of the toluene molecule. By sending an 80-fs Ti:sapphire laser beam through a 2-mm-thick CaF2 plate we show that even moderately broadened laser frequency spectra considerably increase the degree of fragmentation, while it is nearly absent without continuum generation. The measured broadening of the frequency spectra and the known Raman-active vibrational modes of toluene afford an explanation in terms of a stimulated Raman scattering scheme, in which the molecule absorbs large amounts of vibrational energy.

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Language(s): eng - English
 Dates: 2002-01-14
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: Peer
 Degree: -

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Title: Physical Review Letters
  Alternative Title : Phys. Rev. Lett.
Source Genre: Journal
 Creator(s):
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Publ. Info: -
Pages: - Volume / Issue: 88 (2) Sequence Number: 023001 Start / End Page: - 023001 Identifier: ISSN: 0031-9007