English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT
 
 
DownloadE-Mail
 Local TagsRelease HistoryDetailsSummary
  Dynamics of ultrafast photoinduced heterogeneous electron transfer, implications for recent solar energy conversion scenarios

Gundlach, L., Burfeindt, B., Mahrt, J., & Willig, F. (2012). Dynamics of ultrafast photoinduced heterogeneous electron transfer, implications for recent solar energy conversion scenarios. Chemical Physics Letters, 545, 35-39. doi:10.1016/j.cplett.2012.07.011.

Item is

 

show all hide all

Basic

show hide
Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0010-76D5-2 Version Permalink: https://hdl.handle.net/21.11116/0000-0005-16A9-4
Genre: Journal Article

Files

show Files

Locators

show

Creators

show
hide
 Creators:
Gundlach, Lars1, Author
Burfeindt, Bernd2, Author           
Mahrt, Jürgen2, Author           
Willig, Frank2, Author           
Affiliations:
1Dept. of Chemistry and Biochemistry, University of Delaware, Newark, DE 19716, USA, ou_persistent22              
2Theory, Fritz Haber Institute, Max Planck Society, ou_634547              

Content

show
hide
Free keywords: -
 Abstract: The general case of a heterogeneous electron transfer reaction is realized by ultrafast electron transfer
from a photo-excited molecule to a wide continuum of electronic acceptor states. Two different theoretical
model calculations addressing the injection dynamics have recently been presented. The first scenario
predicts a wide energy distribution for the injected electron via excitations of high-energy
vibrational modes in the ionized molecule, whereas the second scenario ascribes the width to thermal
fluctuations. We present experimental data at different temperatures and identify the valid injection scenario
for perylene/TiO2 systems. The results are discussed in view of recent solar energy conversion
scenarios.

Details

show
hide
Language(s): eng - English
 Dates: 2012-05-232012-07-142012-07-05
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1016/j.cplett.2012.07.011
 Degree: -

Event

show

Legal Case

show

Project information

show

Source 1

show
hide
Title: Chemical Physics Letters
  Other : Chem. Phys. Lett.
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: Amsterdam : North-Holland
Pages: - Volume / Issue: 545 Sequence Number: - Start / End Page: 35 - 39 Identifier: ISSN: 0009-2614
CoNE: https://pure.mpg.de/cone/journals/resource/954925389241