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  Ultra-efficient ionization of heavy atoms by intense X-ray free-electron laser pulses

Rudek, B., Son, S.-K., Foucar, L., Epp, S., Erk, B., Hartmann, R., et al. (2012). Ultra-efficient ionization of heavy atoms by intense X-ray free-electron laser pulses. Nature Photonics, 6(12), 858-865. doi:10.1038/nphoton.2012.261.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000E-7847-9 Version Permalink: http://hdl.handle.net/21.11116/0000-0005-1977-A
Genre: Journal Article

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 Creators:
Rudek, Benedikt1, 2, Author
Son, Sang-Kil3, Author
Foucar, L.2, 4, Author
Epp, S.1, 2, Author
Erk, Benjamin1, 2, Author
Hartmann, Robert5, Author
Adolph, Marcus6, Author
Andritschke, Robert7, Author
Aquila, Andrew3, Author
Berrah, Nora8, Author
Bostedt, Christoph9, Author
Bozek, John9, Author
Coppola, Nicola3, Author
Filsinger, Frank10, Author              
Gorke, Hubert11, Author
Gorkhover, Tais6, Author
Graafsma, Heinz12, Author
Gumprecht, Lars3, Author
Hartmann, Andreas5, Author
Hauser, Günter7, 13, Author
Herrmann, Sven7, AuthorHirsemann, Helmut12, AuthorHoll, Peter5, AuthorHömke, André1, 2, AuthorJournel, Loic14, AuthorKaiser, Christian1, AuthorKimmel, Nils13, AuthorKrasniqi, Faton2, 4, AuthorKühnel, Kai-Uwe1, AuthorMatysek, Michael15, AuthorMesserschmidt, Marc9, AuthorMiesner , Danilo7, AuthorMöller, Thomas6, AuthorMoshammer, Robert1, 2, AuthorNagaya, Kiyonobu16, AuthorNilsson, Björn12, AuthorPotdevin, Guillaume12, AuthorPietschner, Daniel13, AuthorReich, Christian5, AuthorRupp, Daniela6, AuthorSchaller, Gerhard7, AuthorSchlichting, Ilme2, 4, AuthorSchmidt, Carlo1, 2, AuthorSchopper, Florian7, AuthorSchorb, Sebastian6, 9, AuthorSchröter, Claus-Dieter1, AuthorSchulz, Joachim3, AuthorSimon, Marc14, AuthorSoltau, Heike5, AuthorStrüder, Lothar2, 13, AuthorUeda, Kiyoshi17, AuthorWeidenspointner, Georg7, 13, AuthorSantra, Robin3, 15, AuthorUllrich, Joachim1, 2, 18, AuthorRudenko, Artem1, 2, 19, AuthorRolles, Daniel2, 4, Author more..
Affiliations:
1Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society, ou_904547              
2Max Planck Advanced Study Group at Center for Free-Electron Laser Science (CFEL), 22607 Hamburg, Germany, ou_persistent22              
3CFEL, Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany, ou_persistent22              
4Max Planck Institute for Medical Research, ou_1125545              
5PNSensor GmbH,, 81739 München, Germany, ou_persistent22              
6Institut für Optik und Atomare Physik, Technische Universität Berlin, 10623 Berlin, Germany, ou_persistent22              
7High Energy Astrophysics, MPI for Extraterrestrial Physics, Max Planck Society, ou_159890              
8Western Michigan University, Physics Department, Kalamazoo, Michigan 49008, USA, ou_persistent22              
9Linac Coherent Light Source, Stanford Linear Accelerator Center (SLAC) National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
10Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
11Forschungszentrum Jülich, Institut Zentrallabor für Elektronik (ZEL), 52428 Jülich, Germany, ou_persistent22              
12Photon Science, DESY, 22607 Hamburg, Germany, ou_persistent22              
13Max-Planck-Institut Halbleiterlabor, 81739 München, Germany, ou_persistent22              
14Laboratoire de Chimie Physique-Matière et Rayonnement, Université Pierre et Marie Curie and Centre national de la recherche scientifique (CNRS), Unité Mixte de Recherche (UMR) 7614, 75231 Paris Cedex 05, France, ou_persistent22              
15Universität Hamburg, 20355 Hamburg, Germany, ou_persistent22              
16Kyoto University, Kyoto 606-8501, Japan, ou_persistent22              
17Tohoku University, Sendai 980-8577, Japan, ou_persistent22              
18Physikalisch-Technische Bundesanstalt, 38116 Braunschweig, Germany, ou_persistent22              
19J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA, ou_persistent22              

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Free keywords: Spectroscopy Fundamental optical physics Ultrafast photonics X-rays
 Abstract: X-ray free-electron lasers provide unique opportunities for exploring ultrafast dynamics and for imaging the structures of complex systems. Understanding the response of individual atoms to intense X-rays is essential for most free-electron laser applications. First experiments have shown that, for light atoms, the dominant interaction mechanism is ionization by sequential electron ejection, where the highest charge state produced is defined by the last ionic state that can be ionized with one photon. Here, we report an unprecedentedly high degree of ionization of xenon atoms by 1.5 keV free-electron laser pulses to charge states with ionization energies far exceeding the photon energy. Comparing ion charge-state distributions and fluorescence spectra with state-of-the-art calculations, we find that these surprisingly high charge states are created via excitation of transient resonances in highly charged ions, and predict resonance enhanced absorption to be a general phenomenon in the interaction of intense X-rays with systems containing high-Z constituents.

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Language(s): eng - English
 Dates: 2012-04-042012-09-172012-11-112012-12
 Publication Status: Published in print
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1038/nphoton.2012.261
 Degree: -

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Title: Nature Photonics
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: -
Pages: - Volume / Issue: 6 (12) Sequence Number: - Start / End Page: 858 - 865 Identifier: ISSN: 1749-4885
CoNE: https://pure.mpg.de/cone/journals/resource/1000000000240270