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  On the determination of absolute vibrational excitation probabilities in molecule-surface scattering: Case study of NO on Au(111).

Cooper, R., Li, Z., Golibrzuch, K., Bartels, C., Rahinov, I., Auerbach, D. J., et al. (2012). On the determination of absolute vibrational excitation probabilities in molecule-surface scattering: Case study of NO on Au(111). The Journal of Chemical Physics, 137(6): 064705. doi:10.1063/1.4738596.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-000E-E7FF-B Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0028-94A4-2
Genre: Journal Article

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 Creators:
Cooper, Russell, Author
Li, Zhisheng, Author
Golibrzuch, Kai, Author
Bartels, Christof, Author
Rahinov, Igor, Author
Auerbach, D. J.1, Author              
Wodtke, A. M.1, Author              
Affiliations:
1Department of Dynamics at Surfaces, MPI for biophysical chemistry, Max Planck Society, ou_578600              

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 Abstract: We describe a method to obtain absolute vibrational excitation probabilities of molecules scattering from a surface based on measurements of the rotational state, scattering angle, and temporal distributions of the scattered molecules and apply this method to the vibrational excitation of NO scattering from Au(111). We report the absolute excitation probabilities to the v = 1 and v = 2 vibrational states, rotational excitation distributions, and final scattering angle distributions for a wide range of incidence energies and surface temperatures. In addition to demonstrating the methodology for obtaining absolute scattering probabilities, these results provide an excellent benchmark for theoretical calculations of molecule-surface scattering.

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Language(s): eng - English
 Dates: 2012-08-102012
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1063/1.4738596
 Degree: -

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Title: The Journal of Chemical Physics
Source Genre: Journal
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Publ. Info: American Chemical Society
Pages: - Volume / Issue: 137 (6) Sequence Number: 064705 Start / End Page: - Identifier: ISSN: 1520-9032
CoNE: https://pure.mpg.de/cone/journals/resource/991042752807952