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  Multi-functional Unit Combining a Fuel Cell and an Enzyme Electro-Membrane Reactor : Concepts, Design, Experiments

Kukula, R., Schultz, T., Schröder, T., Sundmacher, K., & Hasal, P. (2004). Multi-functional Unit Combining a Fuel Cell and an Enzyme Electro-Membrane Reactor: Concepts, Design, Experiments. In CHISA 2004: 16th International Congress of Chemical and Process Engineering (pp. 1138).

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0013-9EE0-9 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-CC7C-8
Genre: Conference Paper

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 Creators:
Kukula, R.1, Author
Schultz, Thorsten2, Author              
Schröder, Torsten2, Author              
Sundmacher, Kai2, 3, Author              
Hasal, P.1, Author
Affiliations:
1Institute of Chemical Technology, PragueDepartment of Chemical Engineering and Center for Nonlinear DynamicsTechnická 516628 Praha 6Czech Republic, ou_persistent22              
2Process Systems Engineering, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, ou_1738151              
3Otto-von-Guericke-Universität Magdeburg, External Organizations, ou_1738156              

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 Abstract: Integrated multi-functional chemical or biochemical reactors have attracted large attention during the last decades due to their interesting operational characteristics, versatility and multi-purpose applicability compared to traditional systems consisting of individual unit operations. The integration of several unit operations and necessary equipment into a single compact unit shortens transport paths, reduces amount of auxiliary media, increases energetic efficiency, reduces amount of wastes produced etc. Here we describe an attempt to integrate the electro-membrane reactor with a fuel cell stack in order to build-up an autonomous (independent of external power source) portable multi-functional unit (MFU). The MFU comprises two sub-units: the first one that generates the electric current (the fuel cell) and the second one that consumes it and simultaneously performs a biotransformation the reactor. The coupling of both sub-units within this kind of MFU is primarily realized by means of the electric current passing through both parts of the system. In our paper we firstly present results of the measurements of the electric behavior of both sub-units: the current voltage curves and the power current characteristic curves of the fuel cell stack under various operating conditions (hydrogen pressure and volumetric flow rate, mode of hydrogen humidification, air flow rate in the cathodes). The current voltage curves and the power characteristic curves of the membrane reactor are also presented using different buffer solutions and various flow rates. The characteristic curves of the fuel cell stack and of the membrane reactor are then compared in order to find appropriate operating regions where both sub-units can be mutually coupled. Residence time distributions in the flow-through compartments of the electro-membrane reactor are also analyzed. An outlook to system design modifications is given based on the conclusions deduced from the experimental results.

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Language(s): eng - English
 Dates: 2004
 Publication Status: Published in print
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 Identifiers: eDoc: 210663
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Title: CHISA 2004 : 16th International Congress of Chemical and Process Engineering
Place of Event: Prague, Czech Republic
Start-/End Date: 2004-08-22 - 2004-08-26

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Title: CHISA 2004 : 16th International Congress of Chemical and Process Engineering
Source Genre: Proceedings
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Pages: CD-ROM Volume / Issue: - Sequence Number: - Start / End Page: 1138 Identifier: -