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  An oscillating liquid-gas reaction with periodic evaporation : nonlinear analysis and experimental results

Zeyer, K. P., Mangold, M., Obertopp, T., & Gilles, E. D. (1999). An oscillating liquid-gas reaction with periodic evaporation: nonlinear analysis and experimental results. Chemical Engineering Science, 54(21), 4845-4851. doi:10.1016/S0009-2509(99)00203-1.

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Datensatz-Permalink: http://hdl.handle.net/11858/00-001M-0000-0013-A287-3 Versions-Permalink: http://hdl.handle.net/11858/00-001M-0000-0027-AC69-6
Genre: Zeitschriftenartikel

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 Urheber:
Zeyer, K. P.1, Autor              
Mangold, M.1, Autor              
Obertopp, T.2, Autor
Gilles, E. D.2, 3, Autor              
Affiliations:
1Process Synthesis and Process Dynamics, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, ou_1738153              
2Universität Stuttgart, ou_persistent22              
3Systems Biology, Max Planck Institute for Dynamics of Complex Technical Systems, Max Planck Society, ou_1738155              

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 Zusammenfassung: In this work we present theoretical and experimental studies of a laboratory scale continuous flow stirred tank reactor (CSTR) in which theiron-(III)-nitrate catalyzed oxidation of ethanol with hydrogen peroxide to ethanal and acetic acid takes place. This reaction displays temperature and concentration oscillations when it is performed in a CSTR. A liquid phase model is known in the literature derived from a more detailed mechanism. This model predicts the location of stationary solutions and bifurcations well, but the calculated reactor temperatures are high above the boiling point of the reaction mixture under certain conditions. Therefore, two different gas/liquid models were developed and compared with the experimental results. © Copyright 2004 Elsevier Science B.V., Amsterdam. All rights reserved. [accessed 2014 March 31st]

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Sprache(n): eng - Englisch
 Datum: 1999
 Publikationsstatus: Im Druck publiziert
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: eDoc: 111976
DOI: 10.1016/S0009-2509(99)00203-1
 Art des Abschluß: -

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Titel: Chemical Engineering Science
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: -
Seiten: - Band / Heft: 54 (21) Artikelnummer: - Start- / Endseite: 4845 - 4851 Identifikator: -