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  Raman study of 2,7-bis(biphenyl-4-yl-)2',7'-ditertbutyl-9,9'-spirobifluorene adsorbed on oxide surfaces

Stähler, J., Hofmann, O. T., Rinke, P., Blumstengel, S., Henneberger, F., Li, Y., et al. (2013). Raman study of 2,7-bis(biphenyl-4-yl-)2',7'-ditertbutyl-9,9'-spirobifluorene adsorbed on oxide surfaces. Chemical Physics Letters, 584, 74-78. doi:10.1016/j.cplett.2013.08.030.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0014-3B38-7 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0014-7638-9
Genre: Journal Article

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Staehler_etal_SP6_ZnO_Raman_DFT_rev.pdf (Any fulltext), 558KB
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2013
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 Creators:
Stähler, Julia1, 2, Author              
Hofmann, Oliver T.3, Author              
Rinke, Patrick3, Author              
Blumstengel, Sylke 4, Author
Henneberger, Fritz4, Author
Li, Yilei2, Author
Heinz, Tony F.2, Author
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Departments of Physics and Electrical Engineering, Columbia University, 538 West 120th Street, New York, New York 10027, USA, ou_persistent22              
3Theory, Fritz Haber Institute, Max Planck Society, ou_634547              
4Institut für Physik, Humboldt-Universität zu Berlin, Newtonstrasse 15, 12489 Berlin, Germany, ou_persistent22              

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 Abstract: We present a systematic non-resonant Raman study of the vibrational properties of the spirobifluorene derivative 2,7-bis(biphenyl-4-yl)-2’,7’-di-tertbutyl-9,9’-spirobifluorene (SP6) on three different substrates: ZnO(000-1), ZnMgO(000-1), and Al2O3(11-20). This investigation of few monolayer coverages is facilitated by the high scattering cross section of this molecule. The vibrational response of SP6 is unaffected by the choice of substrate, showing that the vibrational properties of the molecules remain unchanged by adsorption. Furthermore, we can directly compare the experimental spectra to our density functional theory calculations of the Raman cross sections of SP6 in the gas phase.

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Language(s): eng - English
 Dates: 2013-06-242013-08-102013-08-172013-10-01
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1016/j.cplett.2013.08.030
 Degree: -

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Title: Chemical Physics Letters
  Other : Chem. Phys. Lett.
Source Genre: Journal
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Publ. Info: Amsterdam : North-Holland
Pages: - Volume / Issue: 584 Sequence Number: - Start / End Page: 74 - 78 Identifier: ISSN: 0009-2614
CoNE: https://pure.mpg.de/cone/journals/resource/954925389241