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  Molybdenum-based catalysts for the decomposition of ammonia: In situ X-ray diffraction studies, microstructure, and catalytic properties

Tagliazucca, V., Schlichte, K., Weidenthaler, C., & Schüth, F. (2013). Molybdenum-based catalysts for the decomposition of ammonia: In situ X-ray diffraction studies, microstructure, and catalytic properties. Journal of Catalysis, 305, 277-289. doi:10.1016/j.jcat.2013.05.011.

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 Creators:
Tagliazucca, Valeria1, Author              
Schlichte, Klaus1, Author              
Weidenthaler, Claudia2, Author              
Schüth, Ferdi1, Author              
Affiliations:
1Research Department Schüth, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445589              
2Research Group Weidenthaler, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1950291              

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Free keywords: In situ powder diffraction; Ammonia decomposition; Structure analysis; Molybdenum oxides; Molybdenum nitrides
 Abstract: The ammonia decomposition reaction over molybdenum-based catalysts is an example for the complex influence of different factors, such as phase composition; size of crystalline domains, or defect concentration, on the catalytic behavior of a material. In situ powder diffraction allows the direct analysis of how catalysts change during a reaction with respect to the atomic structure or microstructure in terms of defects or size changes. In this article, the influence of catalyst treatment such as pre-reduction or ball milling on the catalytic properties is discussed in detail.

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Language(s): eng - English
 Dates: 2013-03-112013-06-292013-09-01
 Publication Status: Published in print
 Pages: 13
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1016/j.jcat.2013.05.011
 Degree: -

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Title: Journal of Catalysis
  Abbreviation : J. Catal.
Source Genre: Journal
 Creator(s):
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Publ. Info: Amsterdam : Elsevier
Pages: - Volume / Issue: 305 Sequence Number: - Start / End Page: 277 - 289 Identifier: ISSN: 0021-9517
CoNE: https://pure.mpg.de/cone/journals/resource/954922645027