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  Adapting a Wacker-type catalyst system to the palladium-catalyzed oxidative carbonylation of aliphatic polyols

Doro, F., Winnertz, P., Leitner, W., Prokofieva, A., & Müller, T. E. (2011). Adapting a Wacker-type catalyst system to the palladium-catalyzed oxidative carbonylation of aliphatic polyols. Green Chemistry, 13(2), 292-295. doi:10.1039/C0GC00817F.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-A318-C Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0014-A319-A
Genre: Journal Article

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 Creators:
Doro, Franco1, Author
Winnertz, Patrick1, Author
Leitner, Walter2, 3, Author           
Prokofieva, Angelian1, Author
Müller, Thomas E.1, Author
Affiliations:
1CAT Catalytic Center, ITMC, RWTH Aachen University, Worringerweg 1, Germany , ou_persistent22              
2Service Department Leitner (Technical Labs), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445626              
3Institut für Technische und Makromolekulare Chemie, Technische Chemie und Petrolchemie, RWTH Aachen University, Worringerweg 1, Germany, ou_persistent22              

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 Abstract: Polyols, which can be obtained readily from bio-feedstock, are converted efficiently into their corresponding cyclic carbonates by using a Wacker-type Pd/Mn catalyst system. A fine tuned redox cascade is essential in ensuring a high productivity of the Pd catalyst in the oxidative carbonylation reaction. Turnover numbers up to 784 molproduct/molpalladium were achieved.

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Language(s): eng - English
 Dates: 2010-11-152010-12-152011-01-142011-02-01
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/C0GC00817F
 Degree: -

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Title: Green Chemistry
  Other : Green Chem.
Source Genre: Journal
 Creator(s):
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: 4 Volume / Issue: 13 (2) Sequence Number: - Start / End Page: 292 - 295 Identifier: ISSN: 1463-9262
CoNE: https://pure.mpg.de/cone/journals/resource/954925625301