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  Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure.

Boll, R., Anielski, D., Bostedt, C., Bozek, J. D., Christensen, L., Coffee, R., et al. (2013). Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure. Physical Review A, 88(6): 061402. doi:10.1103/PhysRevA.88.061402.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0014-D121-0 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0027-CEE4-1
Genre: Journal Article

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 Creators:
Boll, R., Author
Anielski, D., Author
Bostedt, C., Author
Bozek, J. D., Author
Christensen, L., Author
Coffee, R., Author
De, S., Author
Decleva, P., Author
Epp, S. W., Author
Erk, B., Author
Foucar, L., Author
Krasnigi, F., Author
Kupper, J., Author
Rouzee, A., Author
Rudek, B., Author
Rudenko, A., Author
Schorb, S., Author
Stapelfeldt, H., Author
Stener, M., Author
Stern, S., Author
Techert, S.1, Author              Trippel, S., AuthorVrakking, M. J. J., AuthorUllrich, J., AuthorRolles, D., Author more..
Affiliations:
1Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for biophysical chemistry, Max Planck Society, ou_578564              

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 Abstract: We demonstrate an experimental method to record snapshot diffraction images of polyatomic gas-phase molecules, which can, in a next step, be used to probe time-dependent changes in the molecular geometry during photochemical reactions with femtosecond temporal and angstrom spatial resolution. Adiabatically laser-aligned 1-ethynyl-4-fluorobenzene (C 8H 5F) molecules were imaged by diffraction of photoelectrons with kinetic energies between 31 and 62 eV, created from core ionization of the fluorine (1s) level by ap80 fs x-ray free-electron-laser pulses. Comparison of the experimental photoelectron angular distributions with density functional theory calculations allows relating the diffraction images to the molecular structure.

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Language(s): eng - English
 Dates: 2013-12-062013-12
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1103/PhysRevA.88.061402
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Title: Physical Review A
Source Genre: Journal
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Pages: 5 Volume / Issue: 88 (6) Sequence Number: 061402 Start / End Page: - Identifier: ISSN: 1050-2947