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  X-Ray Diffraction from Isolated and Strongly Aligned Gas-Phase Molecules with a Free-Electron Laser

Küpper, J., Stern, S., Holmegaard, L., Filsinger, F., Rouzée, A., Rudenko, A., et al. (2014). X-Ray Diffraction from Isolated and Strongly Aligned Gas-Phase Molecules with a Free-Electron Laser. Physical Review Letters, 112(8): 083002. doi:10.1103/PhysRevLett.112.083002.

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PhysRevLett.112.083002.pdf (Verlagsversion), 996KB
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PhysRevLett.112.083002.pdf
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2014
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APS
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 Urheber:
Küpper, Jochen1, 2, 3, 4, 5, Autor           
Stern, Stephan1, 2, Autor
Holmegaard, Lotte1, Autor
Filsinger, Frank4, 5, Autor           
Rouzée, Arnaud6, 7, Autor
Rudenko, Artem5, 8, 9, Autor
Johnsson, Per10, Autor
Martin, Andrew V.1, Autor
Adolph, Marcus11, Autor
Aquila, Andrew1, 12, Autor
Bajt, Saša12, Autor
Barty, Anton1, Autor
Bostedt, Christoph13, Autor
Bozek, John13, Autor
Caleman, Carl1, 14, Autor
Coffee, Ryan13, Autor
Coppola, Nicola1, Autor
Delmas, Tjark1, Autor
Epp, Sascha5, 8, Autor
Erk, Benjamin5, 8, Autor
Foucar, Lutz5, 15, AutorGorkhover, Tais11, AutorGumprecht, Lars1, AutorHartmann, Andreas16, AutorHartmann, Robert16, AutorHauser, Günter17, 18, AutorHoll, Peter16, AutorHömke, Andre5, 8, AutorKimmel, Nils17, AutorKrasniqi, Faton5, 15, AutorKühnel, Kai-Uwe8, AutorMaurer, Jochen19, AutorMesserschmidt, Marc13, AutorMoshammer, Robert5, 8, AutorReich, Christian16, AutorRudek, Benedikt5, 8, AutorSantra, Robin1, 2, 3, AutorSchlichting, Ilme5, 15, AutorSchmidt, Carlo5, AutorSchorb, Sebastian11, AutorSchulz, Joachim1, AutorSoltau, Heike16, AutorSpence, John C. H.20, AutorStarodub, Dmitri20, AutorStrüder, Lothar17, 21, AutorThøgersen, Jan19, AutorVrakking, Marc J. J.6, 7, AutorWeidenspointner, Georg17, 18, AutorWhite, Thomas A.1, AutorWunderer, Cornelia12, AutorMeijer, Gerard4, Autor           Ullrich, Joachim5, 8, AutorStapelfeldt, Henrik19, 22, AutorRolles, Daniel5, 12, 15, AutorChapman, Henry N.1, 2, 3, Autor mehr..
Affiliations:
1Center for Free-Electron-Laser Science (CFEL), DESY, Notkestrasse 85, 22607 Hamburg, Germany, ou_persistent22              
2Hamburg Center for Ultrafast Imaging, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              
3Department of Physics, University of Hamburg, ou_persistent22              
4Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
5Max Planck Advanced Study Group at CFEL, Notkestrasse 85, 22607, ou_persistent22              
6FOM Institute AMOLF, Science Park 104, 1098 XG Amsterdam, Netherlands, ou_persistent22              
7Max-Born-Institute, Max Born Strasse. 2a, 12489 Berlin, Germany, ou_persistent22              
8Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society, ou_904547              
9J. R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA, ou_persistent22              
10Department of Physics, Lund University, P. O. Box 118, 22100 Lund, Sweden, ou_persistent22              
11Technical University of Berlin, 10623 Berlin, Germany, ou_persistent22              
12Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany, ou_persistent22              
13Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA, ou_persistent22              
14Uppsala University, Department of Physics and Astronomy, Box 516, 75120 Uppsala, Sweden, ou_persistent22              
15Max Planck Institute for Medical Research, 69120 Heidelberg, Germany, ou_persistent22              
16PNSensor GmbH, 81739 Munich, Germany, ou_persistent22              
17Max Planck Semiconductor Laboratory, 81739 Munich, Germany, ou_persistent22              
18Max Planck Institute for Extraterrestrial Physics, Max Planck Institute for Extraterrestrial Physics, ou_persistent22              
19Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
20Department of Physics, Arizona State University, Tempe, Arizona 85287, USA, ou_persistent22              
21University of Siegen, Emmy-Noether Campus, Walter Flex Str. 3, 57068 Siegen, Germany, ou_persistent22              
22Interdisciplinary Nanoscience Center (iNANO), Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              

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 Zusammenfassung: We report experimental results on x-ray diffraction of quantum-state-selected and strongly aligned ensembles of the prototypical asymmetric rotor molecule 2,5-diiodobenzonitrile using the Linac Coherent Light Source. The experiments demonstrate first steps toward a new approach to diffractive imaging of distinct structures of individual, isolated gas-phase molecules. We confirm several key ingredients of single molecule diffraction experiments: the abilities to detect and count individual scattered x-ray photons in single shot diffraction data, to deliver state-selected, e.g., structural-isomer-selected, ensembles of molecules to the x-ray interaction volume, and to strongly align the scattering molecules. Our approach, using ultrashort x-ray pulses, is suitable to study ultrafast dynamics of isolated molecules

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Sprache(n): eng - English
 Datum: 2013-07-162014-02-282014-02-28
 Publikationsstatus: Erschienen
 Seiten: 6
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1103/PhysRevLett.112.083002
 Art des Abschluß: -

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Titel: Physical Review Letters
  Andere : Phys. Rev. Lett.
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Woodbury, N.Y. : American Physical Society
Seiten: - Band / Heft: 112 (8) Artikelnummer: 083002 Start- / Endseite: - Identifikator: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1