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  Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure

Boll, R., Anielski, D., Bostedt, C., Bozek, J. D., Christensen, L., Coffee, R., et al. (2013). Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure. Physical Review A, 88(6): 88.061402, pp. 1-5. doi:10.1103/PhysRevA.88.061402.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-8FF9-8 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-8FFA-6
Genre: Journal Article

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 Creators:
Boll, R., Author
Anielski, D., Author
Bostedt, C., Author
Bozek, J. D., Author
Christensen, L., Author
Coffee, R., Author
De, S., Author
Decleva, P., Author
Epp, S. W., Author
Erk, Benjamin1, Author              
Foucar, Lutz1, Author              
Krasniqi, Faton1, Author              
Küpper, J., Author
Rouzée, A., Author
Rudek, Benedikt1, Author              
Rudenko, A., Author
Schorb, S., Author
Stapelfeldt, H., Author
Stener, M., Author
Stern, S., Author
Techert, S., AuthorTrippel, S., AuthorVrakking, M. J. J., AuthorUllrich, J., AuthorRolles, Daniel1, Author               more..
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: We demonstrate an experimental method to record snapshot diffraction images of polyatomic gas-phase molecules, which can, in a next step, be used to probe time-dependent changes in the molecular geometry during photochemical reactions with femtosecond temporal and angstrom spatial resolution. Adiabatically laser-aligned 1-ethynyl-4-fluorobenzene (C8 H5 F) molecules were imaged by diffraction of photoelectrons with kinetic energies between 31 and 62 eV, created from core ionization of the fluorine (1s) level by ≈80 fs x-ray free-electron- laser pulses. Comparison of the experimental photoelectron angular distributions with density functional theory calculations allows relating the diffraction images to the molecular structure

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Language(s): eng - English
 Dates: 2013-08-062013-12-062013-12-06
 Publication Status: Published in print
 Pages: -
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 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevA.88.061402
Other: 7955
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Title: Physical Review A
  Abbreviation : Phys. Rev. A
Source Genre: Journal
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Pages: - Volume / Issue: 88 (6) Sequence Number: 88.061402 Start / End Page: 1 - 5 Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2