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  Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging

Erk, B., Rolles, D., Foucar, L., Rudek, B., Epp, S. W., Cryle, M., et al. (2013). Inner-shell multiple ionization of polyatomic molecules with an intense x-ray free-electron laser studied by coincident ion momentum imaging. Journal of Physics B, 46(16): 164031, pp. 1-12. doi:10.1088/0953-4075/46/16/164031.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-903F-5 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-9040-0
Genre: Journal Article

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JPhysBAtMolOptPhys_46_2013_164031_1 (3).pdf (Any fulltext), 2MB
 
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 Creators:
Erk, Benjamin1, Author              
Rolles, Daniel1, Author              
Foucar, Lutz1, Author              
Rudek, Benedikt1, Author              
Epp, S W, Author
Cryle, Max1, Author              
Bostedt, C, Author
Schorb, S, Author
Bozek, J, Author
Rouzee, A, Author
Hundertmark, A, Author
Marchenko, T, Author
Simon, M, Author
Filsinger, F, Author
Christensen, L, Author
De, S, Author
Trippel, S, Author
Küpper, J, Author
Stapelfeldt, H, Author
Wada, S, Author
Ueda, K, AuthorSwiggers, M, AuthorMesserschmidt, M, AuthorSchröter, C D, AuthorMoshammer, R, AuthorSchlichting, Ilme1, Author              Ullrich, J, AuthorRudenko, A, Author more..
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: The ionization and fragmentation of two selenium containing hydrocarbon molecules, methylselenol (CH3SeH) and ethylselenol (C2H5SeH), by intense (>1017 W cm−2) 5 fs x-ray pulses with photon energies of 1.7 and 2 keV has been studied by means of coincident ion momentum spectroscopy. Measuring charge states and ion kinetic energies, we find signatures of charge redistribution within the molecular environment. Furthermore, by analyzing fragment ion angular correlations, we can determine the laboratory-frame orientation of individual molecules and thus investigate the fragmentation dynamics in the molecular frame. This allows distinguishing protons originating from different molecular sites along with identifying the reaction channels that lead to their emission.

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Language(s): eng - English
 Dates: 2013-03-192013-04-292013-08-132013-08-13
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1088/0953-4075/46/16/164031
Other: 7956
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Title: Journal of Physics B
Source Genre: Journal
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Pages: - Volume / Issue: 46 (16) Sequence Number: 164031 Start / End Page: 1 - 12 Identifier: ISSN: 0953-4075
CoNE: https://pure.mpg.de/cone/journals/resource/954928494403