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  Deep inner-shell multiphoton ionization by intense x-ray free-electron laser pulses

Fukuzawa, H., Son, S.-K., Motomura, K., Mondal, S., Nagaya, K., Wada, S., et al. (2013). Deep inner-shell multiphoton ionization by intense x-ray free-electron laser pulses. Physical Review Letters, 110(17): 173005, pp. 1-5. doi:10.1103/PhysRevLett.110.173005.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-90AE-9 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0019-90AF-7
Genre: Journal Article

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PhysRevLett_110_2013_173005_1.pdf (Any fulltext), 260KB
 
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 Creators:
Fukuzawa, H., Author
Son, S.-K., Author
Motomura, K., Author
Mondal, S., Author
Nagaya, K., Author
Wada, S., Author
Liu, X.-J., Author
Feifel, R., Author
Tachibana, T., Author
Ito, Y., Author
Kimura, M., Author
Sakai, T., Author
Matsunami, K., Author
Hayashita, H., Author
Kajikawa, J., Author
Johnsson, P., Author
Siano, M., Author
Kukk, E., Author
Rudek, Benedikt1, Author              
Erk, Benjamin1, Author              
Foucar, Lutz1, Author              Robert, E., AuthorMiron, C., AuthorTono, K., AuthorInubushi, Y., AuthorHatsui, T., AuthorYabashi, M., AuthorYao, M., AuthorSantra, R., AuthorUeda, K., Author more..
Affiliations:
1Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              

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 Abstract: We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n≥24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers.

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 Dates: 2012-09-232013-04-262013-04-26
 Publication Status: Published in print
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 Rev. Method: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.110.173005
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Pages: - Volume / Issue: 110 (17) Sequence Number: 173005 Start / End Page: 1 - 5 Identifier: ISSN: 0031-9007
CoNE: /journals/resource/954925433406_1