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  Real-Time Manifestation of Strongly Coupled Spin and Charge Order Parameters in Stripe-Ordered La1.75Sr0.25NiO4 Nickelate Crystals Using Time-Resolved Resonant X-Ray Diffraction

Chuang, Y. D., Lee, W. S., Kung, Y. F., Sorini, A. P., Moritz, B., Moore, R. G., et al. (2013). Real-Time Manifestation of Strongly Coupled Spin and Charge Order Parameters in Stripe-Ordered La1.75Sr0.25NiO4 Nickelate Crystals Using Time-Resolved Resonant X-Ray Diffraction. Physical Review Letters, 110(12): 127404. doi:10.1103/PhysRevLett.110.127404.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0019-8E8E-4 Version Permalink: https://hdl.handle.net/11858/00-001M-0000-0028-2E9F-9
Genre: Journal Article

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PhysRevLett.110.127404.pdf (Publisher version), 440KB
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http://dx.doi.org/10.1103/PhysRevLett.110.127404 (Publisher version)
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http://arxiv.org/abs/1302.4522 (Preprint)
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 Creators:
Chuang, Y. D.1, Author
Lee, W. S.2, Author
Kung, Y. F.2, Author
Sorini, A. P.2, 3, Author
Moritz, B.2, 4, 5, Author
Moore, R. G.2, Author
Patthey, L.2, 6, Author
Trigo, M.2, 7, Author
Lu, D. H.8, Author
Kirchmann, P. S.2, Author
Yi, M.2, Author
Krupin, O.9, 10, Author
Langner, M.11, Author
Zhu, Y.11, Author
Zhou, S.Y.11, Author
Reis, D. A.2, 7, Author
Huse, Nils12, Author           
Robinson, J. S.10, Author
Kaindl, R. A.11, Author
Schoenlein, R.W.11, Author
Johnson, S. L.6, AuthorFörst, Michael13, Author           Doering, D.14, AuthorDenes, P.14, AuthorSchlotter, W. F.10, AuthorTurner, J. J.10, AuthorSasagawa, T.15, AuthorHussain, Z.1, AuthorShen, Z. X.2, AuthorDevereaux, T. P.2, Author more..
Affiliations:
1Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              
2SLAC National Accelerator Laboratory, Stanford Institute for Materials and Energy Sciences, Menlo Park, California 94025, USA, ou_persistent22              
3Physics Division, Lawrence Livermore National Laboratory , Livermore, California 94550, USA, ou_persistent22              
4Department of Physics and Astrophysics, University of North Dakota, Grand Forks, North Dakota 58202, USA, ou_persistent22              
5Department of Physics, Northern Illinois University, DeKalb, Illinois 60115, USA, ou_persistent22              
6Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI, Switzerland, ou_persistent22              
7SLAC National Accelerator Laboratory, Stanford PULSE Institute, Menlo Park, California 94025, USA, ou_persistent22              
8Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
9European XFEL GmbH, 22607 Hamburg, Germany, ou_persistent22              
10Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94720, USA, ou_persistent22              
11Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              
12Ultrafast Molecular Dynamics, Research Groups, Max Planck Research Department for Structural Dynamics, Department of Physics, University of Hamburg, External Organizations, ou_2173640              
13Condensed Matter Dynamics Division, Max Planck Research Department for Structural Dynamics, Department of Physics, University of Hamburg, External Organizations, ou_2173637              
14Engineering Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              
15Materials and Structures Laboratory, Tokyo Institute of Technology, Kanagawa 226-8503, Japan, ou_persistent22              

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Free keywords: PACS numbers: 78.70.Ck, 71.27.+a, 78.47.D-, 78.47.J-
 Abstract: We investigate the order parameter dynamics of the stripe-ordered nickelate, La1.75Sr0.25NiO4, using time-resolved resonant x-ray diffraction. In spite of distinct spin and charge energy scales, the two order parameters’ amplitude dynamics are found to be linked together due to strong coupling. Additionally, the vector nature of the spin sector introduces a longer reorientation time scale which is absent in the charge sector. These findings demonstrate that the correlation linking the symmetry-broken states does not unbind during the nonequilibrium process, and the time scales are not necessarily associated with the characteristic energy scales of individual degrees of freedom.

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Language(s): eng - English
 Dates: 2012-08-082013-03-202013-03-22
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.110.127404
arXiv: 1302.4522
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 110 (12) Sequence Number: 127404 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1