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  Investigation of Coking During Dry Reforming of Methane by Means of Thermogravimetry

Tarasov, A., Düdder, H., Mette, K., Kühl, S., Kähler, K., Schlögl, R., et al. (2014). Investigation of Coking During Dry Reforming of Methane by Means of Thermogravimetry. Chemie-Ingenieur-Technik, 86(11), 1916-1924. doi:10.1002/cite.201400092.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0023-E731-9 Version Permalink: http://hdl.handle.net/21.11116/0000-0005-1E3F-5
Genre: Journal Article

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 Creators:
Tarasov, Andrey1, Author              
Düdder, Hendrik2, Author
Mette, Katharina1, Author              
Kühl, Stefanie1, Author              
Kähler, Kevin2, Author
Schlögl, Robert1, Author              
Muhler, Martin2, Author
Behrens, Malte1, 3, Author              
Affiliations:
1Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
2Ruhr-University Bochum, Universitätsstr. 150, 44801 Bochum, Germany, ou_persistent22              
3University of Duisburg-Essen, Faculty of Chemistry and Center for Nanointegration, Duisburg-Essen (CENIDE), Universitätsstr. 7, 45141 Essen, Germany, ou_persistent22              

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Free keywords: CO2 reforming of methane, Nickel catalyst, Thermogravimetry, Carbon deposition
 Abstract: Coking dynamics of Ni-based and Ni-free catalysts were studied in a magnetic suspension thermobalance under methane dry reforming conditions. Ni-rich catalysts undergo strong coking featured with a surface saturation point where the coking rate is drastically reduced. Catalyst resistance towards coking may be enhanced by using noble-metal-based Ni-free precursors or decreasing the Ni content in the catalytic system. The post reaction performed temperature-programmed oxidation experiment of the coked catalyst is diffusion-limited due to large amounts of formed carbon.

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Language(s): eng - English
 Dates: 2014-09-292014-10-092014-11
 Publication Status: Published in print
 Pages: 9
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/cite.201400092
 Degree: -

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Title: Chemie-Ingenieur-Technik
  Other : Chem. Ing. Tech.
Source Genre: Journal
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Publ. Info: Weinheim, Germany : Wiley-VCH
Pages: - Volume / Issue: 86 (11) Sequence Number: - Start / End Page: 1916 - 1924 Identifier: ISSN: 0009-286X
CoNE: https://pure.mpg.de/cone/journals/resource/974740721011