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  Femtosecond electrons probing currents and atomic structure in nanomaterials

Müller, M., Paarmann, A., & Ernstorfer, R. (2014). Femtosecond electrons probing currents and atomic structure in nanomaterials. Nature Communications, 5(10): 5292. doi:10.1038/ncomms6292.

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 Creators:
Müller, Melanie1, Author           
Paarmann, Alexander1, Author           
Ernstorfer, Ralph1, Author           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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Free keywords: Biological sciences Condensed matter Materials science
 Abstract: The investigation of ultrafast electronic and structural dynamics in low-dimensional systems such as nanowires and two-dimensional materials requires femtosecond probes providing high spatial resolution and strong interaction with small volume samples. Low-energy electrons exhibit large scattering cross-sections and high sensitivity to electric fields, but their pronounced dispersion during propagation in vacuum so far prevented their use as femtosecond probe pulses in time-resolved experiments. Here, employing a laser-triggered point-like source of either divergent or collimated electron wave packets, we developed a hybrid approach for femtosecond point projection microscopy and femtosecond low-energy electron diffraction. We investigate ultrafast electric currents in nanowires with sub-100 femtosecond temporal and few 10 nm spatial resolutions, and demonstrate the potential of our approach for studying structural dynamics in crystalline single-layer materials.

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Language(s): eng - English
 Dates: 2014-07-032014-09-172014-10-31
 Publication Status: Published online
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1038/ncomms6292
 Degree: -

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Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
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Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 5 (10) Sequence Number: 5292 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723