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  Cryogenic ion trap vibrational spectroscopy of hydrogen-bonded clusters relevant to atmospheric chemistry

Heine, N., & Asmis, K. R. (2015). Cryogenic ion trap vibrational spectroscopy of hydrogen-bonded clusters relevant to atmospheric chemistry. International Reviews in Physical Chemistry, 34(1), 1-34. doi:10.1080/0144235X.2014.979659.

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 Creators:
Heine, Nadja1, Author              
Asmis, Knut R.1, 2, Author              
Affiliations:
1Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
2Wilhelm-Ostwald-Institut für Physikalische und Theoretische Chemie, Universität Leipzig, ou_persistent22              

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Free keywords: gas phase clusters, vibrational spectroscopy, infrared photodissociation, hydrogen bond, anharmonicity, isomers, cryogenic ion trap
 Abstract: Recent advances in the gas phase vibrational spectroscopy of mass-selected ions are described, highlighting experiments on hydrogen-bonded (HBed) clusters relevant to atmospheric chemistry. The use of cryogenic ion traps in combination with the widely tunable and intense radiation from infrared free electron lasers has allowed for new molecular-level insights into the structure and other properties of HBed clusters. Advances and challenges in the interpretation of their vibrational action spectra, in particular, the importance of considering anharmonic effects, are described and discussed. The advantages of isomer-specific measurements relying exclusively on excitations within the vibrational manifold are also evaluated. The article concludes with an outlook on future challenges and perspectives.

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Language(s): eng - English
 Dates: 2014-09-292014-10-182014-12-062015
 Publication Status: Published in print
 Pages: 34
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1080/0144235X.2014.979659
 Degree: -

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Title: International Reviews in Physical Chemistry
  Other : Int. Rev. Phys. Chem.
Source Genre: Journal
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Publ. Info: Sevenoaks, Kent : Butterworths
Pages: - Volume / Issue: 34 (1) Sequence Number: - Start / End Page: 1 - 34 Identifier: ISSN: 0144-235X
CoNE: https://pure.mpg.de/cone/journals/resource/954925266248