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  Oxidative coupling reactions for the functionalisation of C–H bonds using oxygen

Gulzar, N., Schweitzer-Chaput, B., & Klussmann, M. (2014). Oxidative coupling reactions for the functionalisation of C–H bonds using oxygen. Catalysis Science & Technology, 4(9), 2778-2796. doi:10.1039/c4cy00544a.

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 Creators:
Gulzar, Naeem1, Author              
Schweitzer-Chaput, Bertrand2, Author              
Klussmann, Martin2, Author              
Affiliations:
1Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445585              
2Research Group Klußmann, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445608              

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Free keywords: CARBON-HYDROGEN BONDS; AEROBIC DEHYDROGENATIVE CYCLIZATION; IRON-CATALYZED OXIDATION; BETA-KETO-ESTERS; MOLECULAR-OXYGEN; TERTIARY-AMINES; 4-SUBSTITUTED N,N-DIMETHYLANILINES; PHOTOREDOX CATALYSIS; ATMOSPHERIC OXYGEN; ELECTRON-TRANSFER
 Abstract: Oxidative coupling reactions enable the direct formation of a new bond from two C–H or heteroatom–H bonds without the need for special activating or leaving groups, and are thus interesting in the context of green chemistry. In order to attain high atom economy and sustainability, it is desirable to conduct these reactions catalytically with oxygen or air as terminal oxidant. Here, a representative overview of such reactions is given, illustrating the substrate scope and the variety of catalyst systems. Additionally, mechanisms and general strategies to utilise oxygen in such reactions are discussed.

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Language(s): eng - English
 Dates: 2014-04-282014-06-132014-06-162014-09-01
 Publication Status: Published in print
 Pages: 9
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/c4cy00544a
 Degree: -

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Title: Catalysis Science & Technology
  Other : Catal. Sci. Technol.
Source Genre: Journal
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Publ. Info: Cambridge, England : Royal Chemistry Society
Pages: - Volume / Issue: 4 (9) Sequence Number: - Start / End Page: 2778 - 2796 Identifier: ISSN: 2044-4753
CoNE: https://pure.mpg.de/cone/journals/resource/2044-4753