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  Real-Time Measurement of the Vertical Binding Energy during the Birth of a Solvated Electron

Stähler, J., Deinert, J.-C., Wegkamp, D., Hagen, S., & Wolf, M. (2015). Real-Time Measurement of the Vertical Binding Energy during the Birth of a Solvated Electron. Journal of the American Chemical Society, 137(10), 3520-3524. doi:10.1021/ja511571y.

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 Creators:
Stähler, Julia1, Author           
Deinert, Jan-Christoph1, Author           
Wegkamp, Daniel1, Author           
Hagen, Sebastian1, Author           
Wolf, Martin1, Author           
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1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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 Abstract: Using femtosecond time-resolved two-photon photoelectron spectroscopy, we determine (i) the vertical binding energy (VBE = 0.8 eV) of electrons in the conduction band in supported amorphous solid water (ASW) layers, (ii) the time scale of ultrafast trapping at pre-existing sites (22 fs), and (iii) the initial VBE (1.4 eV) of solvated electrons before significant molecular reorganization sets in. Our results suggest that the excess electron dynamics prior to solvation are representative for bulk ASW.

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Language(s): eng - English
 Dates: 2014-11-172015-01-222015-01-222015-03-18
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/ja511571y
 Degree: -

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Title: Journal of the American Chemical Society
  Other : J. Am. Chem. Soc.
  Abbreviation : JACS
Source Genre: Journal
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Publ. Info: American Chemical Society
Pages: 5 Volume / Issue: 137 (10) Sequence Number: - Start / End Page: 3520 - 3524 Identifier: ISSN: 0002-7863
CoNE: https://pure.mpg.de/cone/journals/resource/954925376870