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  Femtosecond x-ray photoelectron diffraction on gas-phase dibromobenzene molecules

Rolles, D., Boll, R., Adolph, M., Aquila, A., Bostedt, C., Bozek, J. D., et al. (2014). Femtosecond x-ray photoelectron diffraction on gas-phase dibromobenzene molecules. Journal of Physics B, 47(12): 124035. doi:10.1088/0953-4075/47/12/124035.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-B4B6-3 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-B4B8-0
Genre: Journal Article

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 Creators:
Rolles, Daniel1, 2, 3, Author              
Boll , R1, 2, 4, Author
Adolph, M5, Author
Aquila, A6, 7, Author
Bostedt, C8, Author
Bozek, J D8, Author
Chapman, H N6, 9, 10, Author
Coffee, R8, Author
Coppola, N6, 7, Author
Decleva, P11, Author
Delmas, T6, Author
Epp, S. W.1, 4, 12, Author              
Erk, B1, 2, 4, Author
Filsinger, Frank13, 14, Author              
Foucar, L1, 3, Author
Gumprecht, L6, Author
Hömke, A1, 2, 4, Author
Gorkhover, T5, Author
Holmegaard, L6, 15, Author
Johnsson, P16, Author
Kaiser, Ch4, AuthorKrasniqi, F1, 3, 17, Author              Kühnel, K-U4, AuthorMaurer, J15, AuthorMesserschmidt, M8, AuthorMoshammer, R4, AuthorQuevedo, Wilson18, 19, Author              Rajkovic, Ivan18, 20, Author              Rouzée, A21, 22, AuthorRudek, B1, 2, 4, 23, AuthorSchlichting, Ilme1, 3, Author              Schmidt, C1, 2, 4, AuthorSchorb, S5, 8, AuthorSchröter, C D4, AuthorSchulz, J6, 7, AuthorStapelfeldt, H15, AuthorStener, M11, AuthorStern, S6, 9, AuthorTechert, Simone2, 18, 24, Author              Thøgersen, J15, AuthorVrakking, M J J21, 22, AuthorRudenko, A1, 4, 25, AuthorKüpper, Jochen1, 6, 9, 10, 13, Author              Ullrich, J1, 4, 23, Author more..
Affiliations:
1Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany , ou_persistent22              
2Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany , ou_persistent22              
3Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society, ou_1497700              
4Max Planck Institute for Nuclear Physics, 69117 Heidelberg, Germany , ou_persistent22              
5Technische Universität Berlin, 10623 Berlin, Germany , ou_persistent22              
6Center for Free-Electron Laser Science, DESY, 22607 Hamburg, Germany , ou_persistent22              
7European X-ray Free-Electron Laser (XFEL) GmbH, 22761 Hamburg, Germany , ou_persistent22              
8SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA, ou_persistent22              
9Department of Physics, University of Hamburg, 22761 Hamburg, Germany , ou_persistent22              
10The Hamburg Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
11Dipartimento di Scienze Chimiche e Farmaceutiche, Universita di Trieste, 34127 Trieste, Italy , ou_persistent22              
12Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, Luruper Chaussee 149, Geb. 99 (CFEL), 22761 Hamburg, DE, ou_1938288              
13Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
14Bruker AXS GmbH, 76187 Karlsruhe, Germany, ou_persistent22              
15Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
16Department of Physics, Lund University, 22100 Lund, Sweden, ou_persistent22              
17Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, Luruper Chaussee 149, Geb. 99 (CFEL), 22761 Hamburg, DE, ou_1938293              
18Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for biophysical chemistry, Max Planck Society, ou_578564              
19Helmholtz-Zentrum Berlin, 12489 Berlin, Germany, ou_persistent22              
20Paul-Scherrer-Institut, 5232 Villingen, Switzerland, ou_persistent22              
21Max-Born-Institut, 12489 Berlin, Germany, ou_persistent22              
22FOM-Institute AMOLF, 1098 XG Amsterdam, The Netherlands , ou_persistent22              
23Physikalisch-Technische Bundesanstalt (PTB), 38116 Braunschweig, Germany , ou_persistent22              
24Institute of X-ray Physics, Göttingen University, 37077 Göttingen, Germany , ou_persistent22              
25JR MacDonald Laboratory, Kansas State University, Manhattan, KS 66506, USA , ou_persistent22              

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 Abstract: We present time-resolved femtosecond photoelectron momentum images and angular distributions of dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules measured in a near-infrared pump, soft-x-ray probe experiment performed at an x-ray free-electron laser. The observed alignment dependence of the bromine 2p photoelectron angular distributions is compared to density functional theory calculations and interpreted in terms of photoelectron diffraction. While no clear time-dependent effects are observed in the angular distribution of the Br(2p) photoelectrons, other, low-energy electrons show a pronounced dependence on the time delay between the near-infrared laser and the x-ray pulse.

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Language(s): eng - English
 Dates: 2014-01-022014-03-252014-06-102014-06-28
 Publication Status: Published in print
 Pages: 12
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1088/0953-4075/47/12/124035
 Degree: -

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Title: Journal of Physics B
Source Genre: Journal
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Publ. Info: Bristol, UK : IOP Pub.
Pages: - Volume / Issue: 47 (12) Sequence Number: 124035 Start / End Page: - Identifier: ISSN: 0953-4075
CoNE: https://pure.mpg.de/cone/journals/resource/954928494403