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  Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways

Xian, R., Prokhorenko, V., Field, R. L., & Miller, R. J. D. (2015). Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways. Springer Proceedings in Physics, 162, 382-385.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-BE47-B Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-C242-5
Genre: Conference Paper

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Locator:
http://dx.doi.org/10.1007/978-3-319-13242-6_93 (Publisher version)
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 Creators:
Xian, Rui1, Author              
Prokhorenko, Valentyn1, Author              
Field, Ryan L.1, Author
Miller, R. J. Dwayne1, Author              
Affiliations:
1Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288              

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 Abstract: We perform closed- and open-loop coherent control experiments of the photodissociation of triiodide (I3) in ethanol using shaped UV pulses. In the regime where the relative diiodide (I2) yield is excitation-independent, we observe a symmetrical second-order chirp dependence of the I2 yield, and that the I2 production can be controlled within 40 % by varying the second-order chirp of the pump pulse. We show that additional pathways involving higher-lying potential energy surfaces are viable means to explain such observations.

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Language(s): eng - English
 Dates: 2015-01-25
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: Internal
 Identifiers: DOI: 10.1007/978-3-319-13242-6_93
 Degree: -

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Title: 19th International Conference on Ultrafast Phenomena
Place of Event: Okinawa Convention Center, Okinawa, Japan
Start-/End Date: 2014-07-07 - 2014-07-11

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Title: Springer Proceedings in Physics
  Other : Ultrafast Phenomena XIX
Source Genre: Journal
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Publ. Info: Berlin : Springer-Verlag
Pages: - Volume / Issue: 162 Sequence Number: - Start / End Page: 382 - 385 Identifier: ISSN: 0930-8989
CoNE: /journals/resource/110978978742279
ISBN: 978-3-319-13241-9