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  Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure

Boll, R., Anielski, D., Bostedt, C., Bozek, J., Christensen, L., Coffee, R., et al. (2013). Femtosecond photoelectron diffraction on laser-aligned molecules: Towards time-resolved imaging of molecular structure. Physical Review A, 88(6): 061402(R). doi:10.1103/PhysRevA.88.061402.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0024-BB1F-5 Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0027-B55E-9
Genre: Journal Article

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PhysRevA.88.061402.pdf (Publisher version), 2MB
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PhysRevA.88.061402.pdf
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2013
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© American Physical Society
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https://dx.doi.org/10.1103/PhysRevA.88.061402 (Publisher version)
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 Creators:
Boll, R., Author
Anielski, D., Author
Bostedt, C., Author
Bozek, J.D., Author
Christensen, L., Author
Coffee, R., Author
De, S., Author
Decleva, P., Author
Epp, S. W.1, Author              
Erk, B., Author
Foucar, L., Author
Krasniqi, F., Author
Küpper, J., Author
Rouzée, A., Author
Rudek, B., Author
Rudenko, A., Author
Schorb, S., Author
Stapelfeldt, H., Author
Stener, M., Author
Stern, S., Author
Techert, S., AuthorTrippel, S., AuthorVrakking, M.J.J., AuthorUllrich, J., AuthorRolles, D., Author more..
Affiliations:
1Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288              

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Free keywords: PACS numbers: 33.80.Eh, 31.15.es, 33.60.+q
 Abstract: We demonstrate an experimental method to record snapshot diffraction images of polyatomic gas-phase molecules, which can, in a next step, be used to probe time-dependent changes in the molecular geometry during photochemical reactions with femtosecond temporal and angstrom spatial resolution. Adiabatically laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) molecules were imaged by diffraction of photoelectrons with kinetic energies between 31 and 62 eV, created from core ionization of the fluorine (1s) level by ≈80 fs x-ray free-electron-laser pulses. Comparison of the experimental photoelectron angular distributions with density functional theory calculations allows relating the diffraction images to the molecular structure.

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Language(s): eng - English
 Dates: 2013-08-062013-12-062013-12
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: BibTex Citekey: Boll2013
DOI: 10.1103/PhysRevA.88.061402
 Degree: -

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Title: Physical Review A
  Other : Phys. Rev. A
  Other : Physical Review A: Atomic, Molecular, and Optical Physics
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: - Volume / Issue: 88 (6) Sequence Number: 061402(R) Start / End Page: - Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2