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  Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Boll, R., Rouzée, A., Adolph, M., Anielski, D., Aquila, A., Bari, S., et al. (2014). Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules. Faraday Discussions, 171, 57-80. doi:10.1039/C4FD00037D.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0024-BDF9-9 Version Permalink: https://hdl.handle.net/21.11116/0000-0007-1228-8
Genre: Journal Article

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2014
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The Royal Society of Chemistry
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https://dx.doi.org/10.1039/C4FD00037D (Publisher version)
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http://arxiv.org/abs/1407.7782 (Preprint)
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 Creators:
Boll, Rebecca1, 2, 3, Author
Rouzée, Arnaud4, 5, Author
Adolph, Marcus6, Author
Anielski, Denis1, 2, 3, Author
Aquila, Andrew7, 8, Author
Bari, Sadia8, Author
Bomme, Cédric1, Author
Bostedt, Christoph9, Author
Bozek, John D.9, Author
Chapman, Henry N.7, 10, 11, Author
Christensen, Lauge12, Author
Coffee, Ryan9, Author
Coppola, Niccola7, 8, Author
De, Sankar13, 14, Author
Decleva, Piero15, Author
Epp, Sascha W.1, 2, 3, 16, Author           
Erk, Benjamin1, 2, 3, Author
Filsinger, Frank17, Author           
Foucar, Lutz2, 18, Author
Gorkhover, Tais6, Author
Gumprecht, Lars7, AuthorHömke, André1, 2, AuthorHolmegaard, Lotte7, 13, AuthorJohnsson, Per19, AuthorKienitz, Jens S.7, 11, AuthorKierspel, Thomas7, 11, AuthorKrasniqi, Faton2, 18, 20, Author           Kühnel, Kai-Uwe3, AuthorMaurer, Jochen13, AuthorMesserschmidt, Marc9, AuthorMoshammer, Robert2, 3, AuthorMüller, Nele L. M.7, Author           Rudek, Benedikt2, 3, 21, AuthorSavelyev, Evgeny1, 22, AuthorSchlichting, Ilme18, AuthorSchmidt, Carlo2, 3, AuthorScholz, Frank1, AuthorSchorb, Sebastian9, AuthorSchulz, Joachim7, 8, AuthorSeltmann, Jörn1, AuthorStener, Mauro15, AuthorStern, Stephan7, 10, AuthorTechert, Simone1, 2, 22, 23, AuthorThøgersen, Jan13, AuthorTrippel, Sebastian7, AuthorViefhaus, Jens1, AuthorVrakking, Marc4, 5, AuthorStapelfeldt, Henrik13, AuthorKüpper, Jochen2, 7, 10, 11, 17, Author           Ullrich, Joachim2, 3, 21, AuthorRudenko, Artem2, 3, 24, AuthorRolles, Daniel1, 2, 18, Author more..
Affiliations:
1Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany, ou_persistent22              
2Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany, ou_persistent22              
3Max Planck Institute for Nuclear Physics, 69117 Heidelberg, Germany, ou_persistent22              
4Max-Born-Institut, 12489 Berlin, Germany, ou_persistent22              
5FOM-Institute AMOLF, 1098 XG Amsterdam, The Netherlands, ou_persistent22              
6Technische Universität Berlin, 10643 Berlin, Germany, ou_persistent22              
7Center for Free-Electron Laser Science, DESY, 22607 Hamburg, Germany, ou_persistent22              
8European XFEL GmbH, 22761 Hamburg, Germany, ou_persistent22              
9SLAC National Accelerator Laboratory, Menlo Park, USA, ou_persistent22              
10Department of Physics, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
11Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
12Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
13Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
14Saha Institute of Nuclear Physics, 700064 Kolkata, India , ou_persistent22              
15Dipartimento di Scienze Chimiche e Farmaceutiche, Università di Trieste, 34127 Trieste, Italy, ou_persistent22              
16Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288              
17Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
18Max Planck Institute for Medical Research, 69120 Heidelberg, Germany, ou_persistent22              
19Department of Physics, Lund University, 22100 Lund, Sweden, ou_persistent22              
20Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
21Physikalisch-Technische Bundesanstalt (PTB), 38116 Braunschweig, Germany, ou_persistent22              
22Institute of X-ray Physics, University, 37077 Göttingen, Germany, ou_persistent22              
23Max Planck Institute for Biophysical Chemistry, 37077 Göttingen, Germany, ou_persistent22              
24J.R. MacDonald Laboratory, Kansas State University, Manhattan, USA, ou_persistent22              

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Free keywords: Emerging Photon Technologies for Chemical Dynamics
 Abstract: This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump–probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.

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Language(s): eng - English
 Dates: 2014-03-082014-04-032014-07-312014-12-01
 Publication Status: Issued
 Pages: 24
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/C4FD00037D
arXiv: 1407.7782
 Degree: -

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Title: Faraday Discussions
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: London : Royal Society of Chemistry
Pages: - Volume / Issue: 171 Sequence Number: - Start / End Page: 57 - 80 Identifier: ISSN: 1359-6640
CoNE: https://pure.mpg.de/cone/journals/resource/954925269326