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  Global observations of aerosol-cloud-precipitation-climate interactions

Rosenfeld, D., Andreae, M. O., Asmi, A., Chin, M., de Leeuw, G., Donovan, D. P., et al. (2014). Global observations of aerosol-cloud-precipitation-climate interactions. Reviews of Geophysics, 52, 750-808. doi:10.1002/2013RG000441.

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Rosenfeld, Daniel, Autor
Andreae, Meinrat O.1, Autor
Asmi, Ari, Autor
Chin, Mian, Autor
de Leeuw, Gerrit, Autor
Donovan, David P., Autor
Kahn, Ralph, Autor
Kinne, Stefan2, Autor           
Kivekas, Niku, Autor
Kulmala, Markku, Autor
Lau, William, Autor
Schmidt, K. Sebastian, Autor
Suni, Tanja, Autor
Wagner, Thomas1, Autor
Wild, Martin, Autor
Quaas, Johannes, Autor
Affiliations:
1MPI for Chemistry, ou_persistent22              
2Observations and Process Studies, The Atmosphere in the Earth System, MPI for Meteorology, Max Planck Society, ou_913575              

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Schlagwörter: DEEP CONVECTIVE CLOUDS; ASIAN SUMMER MONSOON; CONDENSATION NUCLEI CONCENTRATION; MESOSCALE CELLULAR STRUCTURES; SPECTRAL-RESOLUTION LIDAR; DROPLET EFFECTIVE RADIUS; BOUNDARY-LAYER CLOUDS; BIOMASS BURNING SMOKE; MODIS SATELLITE DATA; OPTICAL DEPTHcloud aerosol interactions; remote sensing; climate change;
 Zusammenfassung: Cloud drop condensation nuclei (CCN) and ice nuclei (IN) particles determine to a large extent cloud microstructure and, consequently, cloud albedo and the dynamic response of clouds to aerosol-induced changes to precipitation. This can modify the reflected solar radiation and the thermal radiation emitted to space. Measurements of tropospheric CCN and IN over large areas have not been possible and can be only roughly approximated from satellite-sensor-based estimates of optical properties of aerosols. Our lack of ability to measure both CCN and cloud updrafts precludes disentangling the effects of meteorology from those of aerosols and represents the largest component in our uncertainty in anthropogenic climate forcing. Ways to improve the retrieval accuracy include multiangle and multipolarimetric passive measurements of the optical signal and multispectral lidar polarimetric measurements. Indirect methods include proxies of trace gases, as retrieved by hyperspectral sensors. Perhaps the most promising emerging direction is retrieving the CCN properties by simultaneously retrieving convective cloud drop number concentrations and updraft speeds, which amounts to using clouds as natural CCN chambers. These satellite observations have to be constrained by in situ observations of aerosol-cloud-precipitation-climate (ACPC) interactions, which in turn constrain a hierarchy of model simulations of ACPC. Since the essence of a general circulation model is an accurate quantification of the energy and mass fluxes in all forms between the surface, atmosphere and outer space, a route to progress is proposed here in the form of a series of box flux closure experiments in the various climate regimes. A roadmap is provided for quantifying the ACPC interactions and thereby reducing the uncertainty in anthropogenic climate forcing.

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Sprache(n): eng - English
 Datum: 2014-12
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: ISI: 000348452000005
DOI: 10.1002/2013RG000441
 Art des Abschluß: -

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Titel: Reviews of Geophysics
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: -
Seiten: - Band / Heft: 52 Artikelnummer: - Start- / Endseite: 750 - 808 Identifikator: ISSN: 8755-1209