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  Ultrabright femtosecond electron sources: perspectives and challenges towards the study of structural dynamics in labile systems

Gao, M., Jean-Ruel, H., Lu, C., Liu, L. C., Marx, A., Cooney, R. R., et al. (2014). Ultrabright femtosecond electron sources: perspectives and challenges towards the study of structural dynamics in labile systems. Proceedings of SPIE, 9198: 91980R. doi:10.1117/12.2062888.

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91980R.pdf (Verlagsversion), 2MB
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2014
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© Society of Photo-Optical Instrumentation Engineers. One print or electronic copy may be made for personal use only. Systematic reproduction and distribution, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper are prohibited.
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externe Referenz:
https://dx.doi.org/10.1117/12.2062888 (Verlagsversion)
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 Urheber:
Gao, Meng1, 2, 3, Autor           
Jean-Ruel, Hubert1, 2, 3, Autor           
Lu, C.2, Autor
Liu, Lai Chung1, 2, 3, Autor           
Marx, Alexander1, 3, Autor           
Cooney, R. R.2, Autor
Jiang, Yifeng1, 2, 3, Autor           
Kassier, Günther1, 2, 3, Autor           
Moriena, Gustavo1, 2, 3, Autor           
Sciaini, Germán1, 2, 3, Autor           
Miller, R. J. Dwayne1, 2, 3, Autor           
Affiliations:
1Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288              
2Departments of Chemistry and Physics, 80 St. George Street, University of Toronto, Toronto, Ontario, M5S 3H6, Canada, ou_persistent22              
3The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany, ou_persistent22              

Inhalt

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Schlagwörter: Ultrafast electron diffraction; structural dynamics; molecular motion
 Zusammenfassung: The advances made in femtosecond electron sources over the last thirty years have been remarkable. In particular, the development of ultrabright femtosecond electron sources has made possible the observation of molecular motion in labile organic materials and it is paving the way towards the study of complex protein systems. The principle of radio frequency (RF) rebunching cavities for the compression of ultrabright electron pulses is presented, alongside with a recent demonstration of its capabilities in capturing the relevant photoinduced dynamics in weakly scattering organic systems. Organic and biological systems can easily decompose or lose crystallinity as a consequence of cumulative heating effects or the formation of side reaction photoproducts. Hence, source brightness plays a crucial role in achieving sufficient signal-to-noise ratio before degradation effects become noticeable on the structural properties of the material. The current brightness of electron sources in addition to the high scattering cross section of keV-MeV electrons have made femtosecond electron diffraction a powerful tool for the study of materials composed by low-Z elements.

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Sprache(n): eng - English
 Datum: 2014-09-05
 Publikationsstatus: Online veröffentlicht
 Seiten: 7
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Interne Begutachtung
 Identifikatoren: DOI: 10.1117/12.2062888
 Art des Abschluß: -

Veranstaltung

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Titel: Ultrafast Nonlinear Imaging and Spectroscopy II
Veranstaltungsort: San Diego, California, United States
Start-/Enddatum: 2014-08-17

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Titel: Proceedings of SPIE
  Andere : Ultrafast Nonlinear Imaging and Spectroscopy II
Genre der Quelle: Zeitschrift
 Urheber:
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Ort, Verlag, Ausgabe: Bellingham, Washington : SPIE
Seiten: - Band / Heft: 9198 Artikelnummer: 91980R Start- / Endseite: - Identifikator: ISSN: 0277-786X
CoNE: https://pure.mpg.de/cone/journals/resource/0277-786X