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  Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules

Boll, R., Rouzée, A., Adolph, M., Anielski, D., Aquila, A., Bari, S., et al. (2014). Imaging molecular structure through femtosecond photoelectron diffraction on aligned and oriented gas-phase molecules. Faraday Discussions, 171, 57-80. doi:10.1039/C4FD00037D.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0025-0820-F Version Permalink: http://hdl.handle.net/11858/00-001M-0000-0025-0821-D
Genre: Journal Article


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Boll, Rebecca1, 2, Author
Rouzée, Arnaud3, 4, Author
Adolph, Marcus5, Author
Anielski , Denis1, 2, Author
Aquila, Andrew6, 7, Author
Bari, Sadia7, Author
Bomme, Cédric1, Author
Bostedt, Christoph8, Author
Bozek, John D.8, Author
Chapman, Henry N.6, 9, 10, Author
Christensen, Lauge11, Author
Coffee, Ryan8, Author
Coppola, Niccola6, 7, Author
De, Sankar12, 13, Author
Decleva, Piero14, Author
Epp, Sascha W.1, 2, 15, Author              
Erk, Benjamin1, 2, Author
Filsinger, Frank16, Author              
Foucar, Lutz2, 17, Author
Gorkhover, Tais5, Author
Gumprecht, Lars6, AuthorHömke, André1, 2, AuthorHolmegaard, Lotte6, 12, AuthorJohnsson, Per18, AuthorKienitz, Jens S.6, 10, AuthorKierspel, Thomas6, 10, AuthorKrasniqi, Faton2, 17, 19, Author              Kühnel, Kai-Uwe, AuthorMaurer, Jochen12, AuthorMesserschmidt, Marc8, AuthorMoshammer, Robert20, Author              Müller, Nele L. M.6, AuthorRudek, Benedikt2, 21, AuthorSavelyev, Evgeny1, 22, AuthorSchlichting, Ilme17, AuthorSchmidt, Carlo2, AuthorScholz, Frank1, AuthorSchorb, Sebastian8, AuthorSchulz, Joachim6, 7, AuthorSeltmann, Jörn1, AuthorStener, Mauro14, AuthorStern, Stephan6, 9, AuthorTechert, Simone1, 2, 22, 23, AuthorThøgersen, Jan12, AuthorTrippel, Sebastian6, AuthorViefhaus, Jens1, AuthorVrakking, Marc3, 4, AuthorStapelfeldt, Henrik12, AuthorKüpper, Jochen2, 6, 9, 10, 16, Author              Ullrich, Joachim2, 21, AuthorRudenko, Artem2, 24, AuthorRolles, Daniel1, 2, 17, Author more..
1Deutsches Elektronen-Synchrotron (DESY), 22607 Hamburg, Germany, ou_persistent22              
2Max Planck Advanced Study Group at CFEL, 22607 Hamburg, Germany, ou_persistent22              
3Max-Born-Institut, 12489 Berlin, Germany, ou_persistent22              
4FOM-Institute AMOLF, 1098 XG Amsterdam, The Netherlands, ou_persistent22              
5Technische Universität Berlin, 10643 Berlin, Germany, ou_persistent22              
6Center for Free-Electron Laser Science, DESY, 22607 Hamburg, Germany, ou_persistent22              
7European XFEL GmbH, 22761 Hamburg, Germany, ou_persistent22              
8SLAC National Accelerator Laboratory, Menlo Park, USA, ou_persistent22              
9Department of Physics, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
10Center for Ultrafast Imaging, University of Hamburg, 22761 Hamburg, Germany, ou_persistent22              
11Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
12Department of Chemistry, Aarhus University, 8000 Aarhus C, Denmark, ou_persistent22              
13Saha Institute of Nuclear Physics, 700064 Kolkata, India , ou_persistent22              
14Dipartimento di Scienze Chimiche e Farmaceutiche, Università di Trieste, 34127 Trieste, Italy, ou_persistent22              
15Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938288              
16Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
17Max Planck Institute for Medical Research, 69120 Heidelberg, Germany, ou_persistent22              
18Department of Physics, Lund University, 22100 Lund, Sweden, ou_persistent22              
19Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
20Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284              
21Physikalisch-Technische Bundesanstalt (PTB), 38116 Braunschweig, Germany, ou_persistent22              
22Institute of X-ray Physics, University, 37077 Göttingen, Germany, ou_persistent22              
23Max Planck Institute for Biophysical Chemistry, 37077 Göttingen, Germany, ou_persistent22              
24J.R. MacDonald Laboratory, Kansas State University, Manhattan, USA, ou_persistent22              


Free keywords: -
 Abstract: This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump–probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.


Language(s): eng - English
 Dates: 2014-07-31
 Publication Status: Published online
 Pages: 24
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1039/C4FD00037D
 Degree: -



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Source 1

Title: Faraday Discussions
Source Genre: Journal
Publ. Info: London : Royal Society of Chemistry
Pages: - Volume / Issue: 171 Sequence Number: - Start / End Page: 57 - 80 Identifier: ISSN: 1359-6640
CoNE: /journals/resource/954925269326