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  A core-level photoionization study of furan

Rennie, E. E., Hergenhahn, U., Kugeler, O., Rüdel, A., Marburger, S., & Bradshaw, A. M. (2002). A core-level photoionization study of furan. Journal of Chemical Physics, 117(14), 6524-6532.

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 Creators:
Rennie, E. E.1, Author
Hergenhahn, U.2, Author              
Kugeler, O.2, Author              
Rüdel, A.3, Author
Marburger, S.3, Author
Bradshaw, A. M.4, Author              
Affiliations:
1Max Planck Society, ou_persistent13              
2Electron Spectroscopy Group (ELSPEC), Max Planck Institute for Plasma Physics, Max Planck Society, ou_1856298              
3Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195; Berlin, Germany, ou_persistent22              
4Office of the Director (DI), Max Planck Institute for Plasma Physics, Max Planck Society, ou_1856325              

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 Abstract: We have measured the vibrationally resolved C 1s photoelectron spectrum of the aromatic heterocycle furan (C4H4O). The vibrational profile appears to be dominated by a low-frequency mode, which shows an unusually high degree of excitation for ionization of the C atoms furthest from the oxygen. Our experimental results are compared with calculations, which reveal that several different vibrational modes participate in the vibrational pattern. A well resolved C 1s satellite spectrum at a photon energy of 335 eV has also been measured, and is compared to previous experimental and theoretical results. In a separate experiment the partial electron yield ("absorption") spectrum has been obtained in the region from just below the C 1s pi* resonance up to the respective ionization thresholds. A new high intensity feature has been identified on the high-energy flank of the C 1s(-1)pi(3b(1))(*) resonance. With the aid of resonant Auger spectroscopy we have tentatively assigned this feature to a Rydberg resonance. We also present the C 1s and O 1s Auger spectra of furan. (C) 2002 American Institute of Physics.

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Language(s): eng - English
 Dates: 2002-10-01
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: eDoc: 21138
ISI: 000178256100018
 Degree: -

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Title: Journal of Chemical Physics
  Alternative Title : J. Chem. Phys.
Source Genre: Journal
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Pages: - Volume / Issue: 117 (14) Sequence Number: - Start / End Page: 6524 - 6532 Identifier: ISSN: 0021-9606