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  Anisotropic Ru3+ 4d5 magnetism in the α-RuCl3 honeycomb system: Susceptibility, specific heat, and zero-field NMR

Majumder, M., Schmidt, M., Rosner, H., Tsirlin, A. A., Yasuoka, H., & Baenitz, M. (2015). Anisotropic Ru3+ 4d5 magnetism in the α-RuCl3 honeycomb system: Susceptibility, specific heat, and zero-field NMR. Physical Review B, 91: 180401, pp. 1-4. doi:10.1103/PhysRevB.91.180401.

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Majumder, M.1, Autor           
Schmidt, M.2, Autor           
Rosner, H.3, Autor           
Tsirlin, A. A.4, Autor           
Yasuoka, H.5, Autor           
Baenitz, M.6, Autor           
Affiliations:
1Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863404              
2Marcus Schmidt, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863415              
3Helge Rosner, Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863450              
4Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863405              
5Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863462              
6Michael Baenitz, Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863471              

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 Zusammenfassung: Hexagonal α-Ru trichloride single crystals exhibit a strong magnetic anisotropy and we show that upon applying fields up to 14 T in the honeycomb plane the successive magnetic order at T1=14K and T2=8K could be completely suppressed, whereas in the perpendicular direction the magnetic order is robust. Furthermore, the field dependence of χ(T) implies coexisting ferro- and antiferromagnetic exchange between in-plane components of Ru3+ spins, whereas for out-of-plane components a strong antiferromagnetic exchange becomes evident. Ru101 zero-field nuclear magnetic resonance in the ordered state evidence a complex (probably noncoplanar chiral) long-range magnetic structure. The large orbital moment on Ru3+ is found in density-functional calculations.

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Sprache(n): eng - English
 Datum: 2015-05-072015-05-07
 Publikationsstatus: Erschienen
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 Identifikatoren: DOI: 10.1103/PhysRevB.91.180401
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Titel: Physical Review B
  Kurztitel : Phys. Rev. B
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Woodbury, NY : American Physical Society
Seiten: - Band / Heft: 91 Artikelnummer: 180401 Start- / Endseite: 1 - 4 Identifikator: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008