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  Anisotropic Ru3+ 4d5 magnetism in the α-RuCl3 honeycomb system: Susceptibility, specific heat, and zero-field NMR

Majumder, M., Schmidt, M., Rosner, H., Tsirlin, A. A., Yasuoka, H., & Baenitz, M. (2015). Anisotropic Ru3+ 4d5 magnetism in the α-RuCl3 honeycomb system: Susceptibility, specific heat, and zero-field NMR. Physical Review B, 91: 180401, pp. 1-4. doi:10.1103/PhysRevB.91.180401.

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Item Permalink: http://hdl.handle.net/11858/00-001M-0000-0026-D09D-5 Version Permalink: http://hdl.handle.net/21.11116/0000-0001-0005-9
Genre: Journal Article

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 Creators:
Majumder, M.1, Author              
Schmidt, M.2, Author              
Rosner, H.3, Author              
Tsirlin, A. A.4, Author              
Yasuoka, H.5, Author              
Baenitz, M.6, Author              
Affiliations:
1Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863404              
2Marcus Schmidt, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863415              
3Helge Rosner, Physics of Correlated Matter, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863450              
4Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863405              
5Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863462              
6Michael Baenitz, Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863471              

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 Abstract: Hexagonal α-Ru trichloride single crystals exhibit a strong magnetic anisotropy and we show that upon applying fields up to 14 T in the honeycomb plane the successive magnetic order at T1=14K and T2=8K could be completely suppressed, whereas in the perpendicular direction the magnetic order is robust. Furthermore, the field dependence of χ(T) implies coexisting ferro- and antiferromagnetic exchange between in-plane components of Ru3+ spins, whereas for out-of-plane components a strong antiferromagnetic exchange becomes evident. Ru101 zero-field nuclear magnetic resonance in the ordered state evidence a complex (probably noncoplanar chiral) long-range magnetic structure. The large orbital moment on Ru3+ is found in density-functional calculations.

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Language(s): eng - English
 Dates: 2015-05-072015-05-07
 Publication Status: Published in print
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Method: -
 Identifiers: DOI: 10.1103/PhysRevB.91.180401
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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: - Volume / Issue: 91 Sequence Number: 180401 Start / End Page: 1 - 4 Identifier: ISSN: 1098-0121
CoNE: /journals/resource/954925225008